New insights on mercury abatement and modeling in a full-scale municipal solid waste incineration flue gas treatment unit

Copyright © 2020 Elsevier Ltd. All rights reserved.

Détails bibliographiques
Publié dans:Waste management (New York, N.Y.). - 1999. - 113(2020) vom: 15. Juli, Seite 270-279
Auteur principal: Romero, Lina M (Auteur)
Autres auteurs: Lyczko, Nathalie, Nzihou, Ange, Antonini, Gérard, Moreau, Eric, Richardeau, Hubert, Coste, Christophe, Madoui, Saïd, Durécu, Sylvain
Format: Article en ligne
Langue:English
Publié: 2020
Accès à la collection:Waste management (New York, N.Y.)
Sujets:Journal Article Equilibrium and kinetics modelling Full-scale parametric study Mercury removal efficiency Mercury transformation mechanisms Solid waste incineration Air Pollutants Solid Waste Mercury FXS1BY2PGL
LEADER 01000caa a22002652c 4500
001 NLM311383580
003 DE-627
005 20250227111300.0
007 cr uuu---uuuuu
008 231225s2020 xx |||||o 00| ||eng c
024 7 |a 10.1016/j.wasman.2020.06.003  |2 doi 
028 5 2 |a pubmed25n1037.xml 
035 |a (DE-627)NLM311383580 
035 |a (NLM)32559697 
035 |a (PII)S0956-053X(20)30313-5 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Romero, Lina M  |e verfasserin  |4 aut 
245 1 0 |a New insights on mercury abatement and modeling in a full-scale municipal solid waste incineration flue gas treatment unit 
264 1 |c 2020 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Completed 14.07.2020 
500 |a Date Revised 14.07.2020 
500 |a published: Print-Electronic 
500 |a Citation Status MEDLINE 
520 |a Copyright © 2020 Elsevier Ltd. All rights reserved. 
520 |a Modeling approaches are generally used to describe mercury transformations in a single step of flue gas treatment processes. However, less attention has been given to the interactions between the different process stages. Accordingly, the mercury removal performance of a full-scale solid waste incineration plant, equipped with a dry flue gas treatment line was investigated using two complementary modeling strategies: a thermochemical equilibrium approach to study the mercury transformation mechanisms and speciation in the flue gas, and a kinetic approach to describe the mercury adsorption process. The modeling observations were then compared to real-operation full-scale data. Considering the typical flue gas composition of waste incineration facilities (high concentrations of HCl compared to Hg), it was found that a process temperature decrease results in better mercury removal efficiencies, associated with a higher oxidation extent of Hg in HgCl2, and the enhancement of the sorbent capacity. Improvements can also be attained by increasing the sorbent injection rate to the process, or the solid/gas separation cycles. An empirical correlation to predict the mercury removal efficiency from the main operating parameters of dry flue gas treatment units was proposed, representing a useful tool for waste incineration facilities. The presented modeling approach proved to be suitable to evaluate the behavior of full-scale gas treatment units, and properly select the most adequate adjustments in operating parameters, in order to respect the increasingly constraining mercury emissions regulations 
650 4 |a Journal Article 
650 4 |a Equilibrium and kinetics modelling 
650 4 |a Full-scale parametric study 
650 4 |a Mercury removal efficiency 
650 4 |a Mercury transformation mechanisms 
650 4 |a Solid waste incineration 
650 7 |a Air Pollutants  |2 NLM 
650 7 |a Solid Waste  |2 NLM 
650 7 |a Mercury  |2 NLM 
650 7 |a FXS1BY2PGL  |2 NLM 
700 1 |a Lyczko, Nathalie  |e verfasserin  |4 aut 
700 1 |a Nzihou, Ange  |e verfasserin  |4 aut 
700 1 |a Antonini, Gérard  |e verfasserin  |4 aut 
700 1 |a Moreau, Eric  |e verfasserin  |4 aut 
700 1 |a Richardeau, Hubert  |e verfasserin  |4 aut 
700 1 |a Coste, Christophe  |e verfasserin  |4 aut 
700 1 |a Madoui, Saïd  |e verfasserin  |4 aut 
700 1 |a Durécu, Sylvain  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Waste management (New York, N.Y.)  |d 1999  |g 113(2020) vom: 15. Juli, Seite 270-279  |w (DE-627)NLM098197061  |x 1879-2456  |7 nnas 
773 1 8 |g volume:113  |g year:2020  |g day:15  |g month:07  |g pages:270-279 
856 4 0 |u http://dx.doi.org/10.1016/j.wasman.2020.06.003  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_350 
951 |a AR 
952 |d 113  |j 2020  |b 15  |c 07  |h 270-279