The impact of lime additions on mercury dynamics in stream chemistry and macroinvertebrates : a comparison of watershed and direct stream addition management strategies

Acid deposition has declined across eastern North America and northern Europe due to reduced emissions of sulfur and nitrogen oxides. Ecosystem recovery has been slow with limited improvement in surface water chemistry. Delayed recovery has encouraged acid-neutralization strategies to accelerate rec...

Ausführliche Beschreibung

Bibliographische Detailangaben
Veröffentlicht in:Ecotoxicology (London, England). - 1992. - 29(2020), 10 vom: 18. Dez., Seite 1627-1643
1. Verfasser: Millard, Geoffrey D (VerfasserIn)
Weitere Verfasser: Riva-Murray, Karen, Burns, Douglas A, Montesdeoca, Mario R, Driscoll, Charles T
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Ecotoxicology (London, England)
Schlagworte:Journal Article Calcium carbonate Macro-invertebrates Mercury Methylmercury Remediation Stream Methylmercury Compounds Water Pollutants, Chemical Carbon mehr... 7440-44-0 FXS1BY2PGL
LEADER 01000caa a22002652c 4500
001 NLM311359531
003 DE-627
005 20250227110821.0
007 cr uuu---uuuuu
008 231225s2020 xx |||||o 00| ||eng c
024 7 |a 10.1007/s10646-020-02224-1  |2 doi 
028 5 2 |a pubmed25n1037.xml 
035 |a (DE-627)NLM311359531 
035 |a (NLM)32557267 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Millard, Geoffrey D  |e verfasserin  |4 aut 
245 1 4 |a The impact of lime additions on mercury dynamics in stream chemistry and macroinvertebrates  |b a comparison of watershed and direct stream addition management strategies 
264 1 |c 2020 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Completed 18.11.2020 
500 |a Date Revised 18.11.2020 
500 |a published: Print-Electronic 
500 |a Citation Status MEDLINE 
520 |a Acid deposition has declined across eastern North America and northern Europe due to reduced emissions of sulfur and nitrogen oxides. Ecosystem recovery has been slow with limited improvement in surface water chemistry. Delayed recovery has encouraged acid-neutralization strategies to accelerate recovery of impaired biological communities. Lime application has been shown to increase pH and dissolved organic carbon (DOC), which could also drive increased mobilization of mercury (Hg) to surface waters. A four-year study was conducted within Honnedaga Lake's watershed in the Adirondack region of New York to compare the effects of watershed and direct channel lime additions on Hg in stream water and macroinvertebrates. All treatments sharply increased stream pH and DOC concentrations, but large differences in the duration of impacts were apparent. The watershed treatment resulted in multi-year increases in concentrations and loads of total Hg (150%; 390%), DOC (190%; 350%) and nutrients, whereas total Hg and DOC increased for short periods (72-96 h) after channel treatments. No response of Hg in macroinvertebrates was evident following the watershed treatment, but a potential short-term and spatially constrained increase occurred after the channel treatment. Our observations indicate that both treatment approaches mobilize Hg, but that direct channel liming mobilizes considerably less than watershed liming over any period longer than a few days. During the final study year, increased methyl Hg concentrations were observed across reference and treated streams, which may reflect an extended dry period, highlighting that climate variation may also affect Hg dynamics 
650 4 |a Journal Article 
650 4 |a Calcium carbonate 
650 4 |a Macro-invertebrates 
650 4 |a Mercury 
650 4 |a Methylmercury 
650 4 |a Remediation 
650 4 |a Stream 
650 7 |a Methylmercury Compounds  |2 NLM 
650 7 |a Water Pollutants, Chemical  |2 NLM 
650 7 |a Carbon  |2 NLM 
650 7 |a 7440-44-0  |2 NLM 
650 7 |a Mercury  |2 NLM 
650 7 |a FXS1BY2PGL  |2 NLM 
700 1 |a Riva-Murray, Karen  |e verfasserin  |4 aut 
700 1 |a Burns, Douglas A  |e verfasserin  |4 aut 
700 1 |a Montesdeoca, Mario R  |e verfasserin  |4 aut 
700 1 |a Driscoll, Charles T  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Ecotoxicology (London, England)  |d 1992  |g 29(2020), 10 vom: 18. Dez., Seite 1627-1643  |w (DE-627)NLM098212214  |x 1573-3017  |7 nnas 
773 1 8 |g volume:29  |g year:2020  |g number:10  |g day:18  |g month:12  |g pages:1627-1643 
856 4 0 |u http://dx.doi.org/10.1007/s10646-020-02224-1  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_65 
912 |a GBV_ILN_350 
951 |a AR 
952 |d 29  |j 2020  |e 10  |b 18  |c 12  |h 1627-1643