Perovskite Single-Crystal Microwire-Array Photodetectors with Performance Stability beyond 1 Year

© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 28 vom: 01. Juli, Seite e2001998
1. Verfasser: Li, Shun-Xin (VerfasserIn)
Weitere Verfasser: Xu, Yi-Shi, Li, Cheng-Long, Guo, Qi, Wang, Gong, Xia, Hong, Fang, Hong-Hua, Shen, Liang, Sun, Hong-Bo
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article flexible photodetectors long-term stability microwires organic-inorganic hybrid perovskites
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520 |a Compared with thin-film morphology, 1D perovskite structures such as micro/nanowires with fewer grain boundaries and lower defect density are very suitable for high-performance photodetectors with higher stability. Although the stability of perovskite microwire-based photodetectors has been substantially enhanced in comparison with that of photodetectors based on thin-film morphology, practical applications require further improvements to the stability before implementation. In this study, a template-assisted method is developed to prepare methylammonium lead bromide (MAPbBr3 ) micro/nanowire structures, which are encapsulated in situ by a protective hydrophobic molecular layer. The combination of the protective layer, high crystalline quality, and highly ordered microstructures significantly improve the stability of the MAPbBr3 single-crystal microwire arrays. Consequently, these MAPbBr3 single-crystal microwire-array-based photodetectors exhibit significant long-term stability, maintaining 96% of the initial photocurrent after 1 year without further encapsulation. The lifetime of such photodetectors is hence approximately four times longer than that of the most stable previously reported perovskite micro/nanowire-based photodetector; this is thought to be the most stable perovskite photodetector reported thus far. Furthermore, this work should contribute further toward the realization of perovskite 1D structures with long-term stability 
650 4 |a Journal Article 
650 4 |a flexible photodetectors 
650 4 |a long-term stability 
650 4 |a microwires 
650 4 |a organic-inorganic hybrid perovskites 
700 1 |a Xu, Yi-Shi  |e verfasserin  |4 aut 
700 1 |a Li, Cheng-Long  |e verfasserin  |4 aut 
700 1 |a Guo, Qi  |e verfasserin  |4 aut 
700 1 |a Wang, Gong  |e verfasserin  |4 aut 
700 1 |a Xia, Hong  |e verfasserin  |4 aut 
700 1 |a Fang, Hong-Hua  |e verfasserin  |4 aut 
700 1 |a Shen, Liang  |e verfasserin  |4 aut 
700 1 |a Sun, Hong-Bo  |e verfasserin  |4 aut 
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773 1 8 |g volume:32  |g year:2020  |g number:28  |g day:01  |g month:07  |g pages:e2001998 
856 4 0 |u http://dx.doi.org/10.1002/adma.202001998  |3 Volltext 
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