Highly Thermotolerant Metal Halide Perovskite Solids

© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 28 vom: 27. Juli, Seite e2002495
1. Verfasser: Lian, Huiwang (VerfasserIn)
Weitere Verfasser: Li, Yang, Sharafudeen, Kaniyarakkal, Zhao, Weiren, Krishnan, Gopi R, Zhang, Shaoan, Qiu, Jianrong, Huang, Kai, Han, Gang
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article enhanced stability heterogeneous interfacial method solid-state metal halide perovskites superior thermotolerance
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520 |a By virtue of their narrow emission bands, near-unity quantum yield, and low fabrication cost, metal halide perovskites hold great promise in numerous aspects of optoelectronic applications, including solid-state lighting, lasing, and displays. Despite such promise, the poor temperature tolerance and suboptimal quantum yield of the existing metal halide perovskites in their solid state have severely limited their practical applications. Here, a straightforward heterogeneous interfacial method to develop superior thermotolerant and highly emissive solid-state metal halide perovskites is reported and their use as long-lasting high-temperature and high-input-power durable solid-state light-emitting diodes is illustrated. It is found that the resultant materials can well maintain their superior quantum efficiency after heating at a temperature over 150 °C for up to 22 h. A white light-emitting diode (w-LED) constructed from the metal halide perovskite solid exhibits superior temperature sustainable lifetime over 1100 h. The w-LED also displays a highly durable high-power-driving capability, and its working current can go up to 300 mA. It is believed that such highly thermotolerant metal halide perovskites will unleash the possibility of a wide variety of high-power and high-temperature solid-state lighting, lasing, and display devices that have been limited by existing methods 
650 4 |a Journal Article 
650 4 |a enhanced stability 
650 4 |a heterogeneous interfacial method 
650 4 |a solid-state metal halide perovskites 
650 4 |a superior thermotolerance 
700 1 |a Li, Yang  |e verfasserin  |4 aut 
700 1 |a Sharafudeen, Kaniyarakkal  |e verfasserin  |4 aut 
700 1 |a Zhao, Weiren  |e verfasserin  |4 aut 
700 1 |a Krishnan, Gopi R  |e verfasserin  |4 aut 
700 1 |a Zhang, Shaoan  |e verfasserin  |4 aut 
700 1 |a Qiu, Jianrong  |e verfasserin  |4 aut 
700 1 |a Huang, Kai  |e verfasserin  |4 aut 
700 1 |a Han, Gang  |e verfasserin  |4 aut 
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773 1 8 |g volume:32  |g year:2020  |g number:28  |g day:27  |g month:07  |g pages:e2002495 
856 4 0 |u http://dx.doi.org/10.1002/adma.202002495  |3 Volltext 
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