Flexible and Self-Powered Photodetector Arrays Based on All-Inorganic CsPbBr3 Quantum Dots

© 2020 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 22 vom: 14. Juni, Seite e2000004
1. Verfasser: Shen, Kai (VerfasserIn)
Weitere Verfasser: Xu, Hao, Li, Xiao, Guo, Jian, Sathasivam, Sanjayan, Wang, Mingqing, Ren, Aobo, Choy, Kwang Leong, Parkin, Ivan P, Guo, Zhengxiao, Wu, Jiang
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article flexible devices perovskites photodetector arrays self-powered devices
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520 |a Flexible devices are garnering substantial interest owing to their potential for wearable and portable applications. Here, flexible and self-powered photodetector arrays based on all-inorganic perovskite quantum dots (QDs) are reported. CsBr/KBr-mediated CsPbBr3 QDs possess improved surface morphology and crystallinity with reduced defect densities, in comparison with the pristine ones. Systematic material characterizations reveal enhanced carrier transport, photoluminescence efficiency, and carrier lifetime of the CsBr/KBr-mediated CsPbBr3 QDs. Flexible photodetector arrays fabricated with an optimum CsBr/KBr treatment demonstrate a high open-circuit voltage of 1.3 V, responsivity of 10.1 A W-1 , specific detectivity of 9.35 × 1013 Jones, and on/off ratio up to ≈104 . Particularly, such performance is achieved under the self-powered operation mode. Furthermore, outstanding flexibility and electrical stability with negligible degradation after 1600 bending cycles (up to 60°) are demonstrated. More importantly, the flexible detector arrays exhibit uniform photoresponse distribution, which is of much significance for practical imaging systems, and thus promotes the practical deployment of perovskite products 
650 4 |a Journal Article 
650 4 |a flexible devices 
650 4 |a perovskites 
650 4 |a photodetector arrays 
650 4 |a self-powered devices 
700 1 |a Xu, Hao  |e verfasserin  |4 aut 
700 1 |a Li, Xiao  |e verfasserin  |4 aut 
700 1 |a Guo, Jian  |e verfasserin  |4 aut 
700 1 |a Sathasivam, Sanjayan  |e verfasserin  |4 aut 
700 1 |a Wang, Mingqing  |e verfasserin  |4 aut 
700 1 |a Ren, Aobo  |e verfasserin  |4 aut 
700 1 |a Choy, Kwang Leong  |e verfasserin  |4 aut 
700 1 |a Parkin, Ivan P  |e verfasserin  |4 aut 
700 1 |a Guo, Zhengxiao  |e verfasserin  |4 aut 
700 1 |a Wu, Jiang  |e verfasserin  |4 aut 
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773 1 8 |g volume:32  |g year:2020  |g number:22  |g day:14  |g month:06  |g pages:e2000004 
856 4 0 |u http://dx.doi.org/10.1002/adma.202000004  |3 Volltext 
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