In Situ Coating Graphdiyne for High-Energy-Density and Stable Organic Cathodes

© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 14 vom: 16. Apr., Seite e2000140
1. Verfasser: Li, Liang (VerfasserIn)
Weitere Verfasser: Zuo, Zicheng, Wang, Fan, Gao, Jingchi, Cao, Anmin, He, Feng, Li, Yuliang
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article graphdiyne lithium-ion batteries organic cathodes sodium-ion batteries
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520 |a The preparation of organic small-molecule cathodes is simple and low-cost; however, their low conductivity and molecular dissolution are two key issues that mean their energy density and power performance are far lower than those of inorganic batteries, thus hindering their practical application. To develop an effective coating technology is the key to obtain high-performance organic batteries. A general method of in situ weaving all-carbon graphdiyne nanocoatings is demonstrated. The graphdiyne can be conformally weaved on organic particles under mild conditions so that the conductivity is increased and the dissolution is suppressed. After weaving graphdiyne nanocoat, the active mass of the small-molecule organic cathodes rise to 93%, thus delivering a higher energy density of 310 W h kg-1 than previously reported, and the power performance and long-term stability are greatly improved. Additionally, this method shows great potential to become the crucial technology for fabricating organic batteries with energy density close to prevailing lithium-ion batteries 
650 4 |a Journal Article 
650 4 |a graphdiyne 
650 4 |a lithium-ion batteries 
650 4 |a organic cathodes 
650 4 |a sodium-ion batteries 
700 1 |a Zuo, Zicheng  |e verfasserin  |4 aut 
700 1 |a Wang, Fan  |e verfasserin  |4 aut 
700 1 |a Gao, Jingchi  |e verfasserin  |4 aut 
700 1 |a Cao, Anmin  |e verfasserin  |4 aut 
700 1 |a He, Feng  |e verfasserin  |4 aut 
700 1 |a Li, Yuliang  |e verfasserin  |4 aut 
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