Solution-Processed Centimeter-Scale Highly Aligned Organic Crystalline Arrays for High-Performance Organic Field-Effect Transistors

© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 12 vom: 06. März, Seite e1908388
1. Verfasser: Duan, Shuming (VerfasserIn)
Weitere Verfasser: Wang, Tao, Geng, Bowen, Gao, Xiong, Li, Chenguang, Zhang, Jing, Xi, Yue, Zhang, Xiaotao, Ren, Xiaochen, Hu, Wenping
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article organic crystalline films organic semiconductors patterning solution process
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520 |a Solution-printed organic single-crystalline films hold great potential for achieving low-cost manufacturing of large-area and flexible electronics. For practical applications, organic field-effect transistor arrays must exhibit high performance and small device-to-device variation. However, scalable fabrication of highly aligned organic crystalline arrays is rather difficult due to the lack of control over the crystallographic orientation, crystal uniformity, and thickness. Here, a facile solution-printing method to fabricate centimeter-sized highly aligned organic crystalline arrays with a thickness of a few molecular layers is reported. In this study, the solution shearing technique is used to produce large-area, organic highly crystalline thin films. Water-soluble ink is printed on the hydrophobic surface of organic crystalline films, to selectively protect it, followed by etching. It is shown that the addition of a surfactant dramatically changes the fluid drying dynamics and increases the contact line friction of the aqueous solution to the underlying nonwetting organic crystalline film. As a result, centimeter-scale highly aligned organic crystalline arrays are successfully prepared on different substrates. The devices based on organic crystalline arrays show good performance and uniformity. This study demonstrates that solution printing is close to industrial application and also expands its applicability to various printed flexible electronics 
650 4 |a Journal Article 
650 4 |a organic crystalline films 
650 4 |a organic semiconductors 
650 4 |a patterning 
650 4 |a solution process 
700 1 |a Wang, Tao  |e verfasserin  |4 aut 
700 1 |a Geng, Bowen  |e verfasserin  |4 aut 
700 1 |a Gao, Xiong  |e verfasserin  |4 aut 
700 1 |a Li, Chenguang  |e verfasserin  |4 aut 
700 1 |a Zhang, Jing  |e verfasserin  |4 aut 
700 1 |a Xi, Yue  |e verfasserin  |4 aut 
700 1 |a Zhang, Xiaotao  |e verfasserin  |4 aut 
700 1 |a Ren, Xiaochen  |e verfasserin  |4 aut 
700 1 |a Hu, Wenping  |e verfasserin  |4 aut 
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773 1 8 |g volume:32  |g year:2020  |g number:12  |g day:06  |g month:03  |g pages:e1908388 
856 4 0 |u http://dx.doi.org/10.1002/adma.201908388  |3 Volltext 
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