Synergetic adsorption and photo-Fenton degradation of methylene blue by ZnFe2O4/SiO2 magnetic double-mesoporous-shelled hollow spheres
Adsorption and Fenton technologies have been widely employed to deal with wastewater. ZnFe2O4/SiO2 magnetic double-mesoporous-shelled hollow spheres (MDSHSs) were feasibly synthesized by a solvothermal method. The as-synthesized MDSHSs show excellent adsorption and selectivity for methylene blue (MB...
| Veröffentlicht in: | Environmental technology. - 1993. - 42(2021), 20 vom: 01. Aug., Seite 3218-3230 |
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| Format: | Online-Aufsatz |
| Sprache: | English |
| Veröffentlicht: |
2021
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| Zugriff auf das übergeordnete Werk: | Environmental technology |
| Schlagworte: | Journal Article ZnFe2O4/SiO2 adsorption magnetic property photo-Fenton porous materials Silicon Dioxide 7631-86-9 Methylene Blue T42P99266K |
| Zusammenfassung: | Adsorption and Fenton technologies have been widely employed to deal with wastewater. ZnFe2O4/SiO2 magnetic double-mesoporous-shelled hollow spheres (MDSHSs) were feasibly synthesized by a solvothermal method. The as-synthesized MDSHSs show excellent adsorption and selectivity for methylene blue (MB), which it took about only 1 min to reach the adsorption equilibrium. About 50% MB was removed by adsorption, and other 50% MB was degraded under further photo-Fenton process. Effects of experimental conditions on the adsorption and photo-Fenton process were investigated. The mechanisms of MDSHSs formation and photo-Fenton process were proposed. Total organic carbon (TOC) reduction reached as high as 90% with 60 mg/L of MB for 90 min. The experimental results indicated that MDSHSs exhibit a remarkable adsorption and catalytic activity for photo-Fenton process in a wide pH range of 3.3-11.0. Simultaneously, the composite shows an excellent stability and reusability |
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| Beschreibung: | Date Completed 12.08.2021 Date Revised 12.08.2021 published: Print-Electronic Citation Status MEDLINE |
| ISSN: | 1479-487X |
| DOI: | 10.1080/09593330.2020.1725142 |