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231225s2020 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201902724
|2 doi
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|a pubmed24n1012.xml
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|a DE-627
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|a eng
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| 100 |
1 |
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|a Liu, Xuejun
|e verfasserin
|4 aut
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| 245 |
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|a Novel Organophosphate-Derived Dual-Layered Interface Enabling Air-Stable and Dendrite-Free Lithium Metal Anode
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|c 2020
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Completed 17.01.2020
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Lithium (Li) metal, as a promising candidate for next-generation energy storage systems, suffers from an extremely unstable interface that is prone to crack, causing serious corrosion of Li metal and dendrite growth. To address this, a novel dual-layered interface on the Li metal anode is reported, which is featured with organics (COPO3 , (CO)2 PO2 , and (CO)3 PO) on the top and inorganics (Li3 PO4 ) at the bottom. The flexible organic layer with reduced Young's modulus (≈550 MPa) contributes to maintain structural integrity, while the rigid inorganic layer with improved Young's modulus of ≈12 GPa is beneficial to suppress the Li dendrite growth. Accordingly, the protected Li is stabilized to maintain successive electrodeposition over 800 cycles of plating/stripping process at a current density of 2 mA cm-2 . Furthermore, the uniform dual-layered interface tends to prevent the corrosion of air to Li metal, exhibiting almost the same performance as the Li metal treated in the inert atmosphere
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|a Journal Article
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|a air-stable anodes
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|a dual-layered interfaces
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| 650 |
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|a lithium metal batteries
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| 700 |
1 |
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|a Liu, Jie
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Qian, Tao
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chen, Hongli
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yan, Chenglin
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 32(2020), 2 vom: 10. Jan., Seite e1902724
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:32
|g year:2020
|g number:2
|g day:10
|g month:01
|g pages:e1902724
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|u http://dx.doi.org/10.1002/adma.201902724
|3 Volltext
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