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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.9b03116
|2 doi
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|a pubmed24n1011.xml
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|a (NLM)31738565
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|a DE-627
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|c DE-627
|e rakwb
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|a eng
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|a Alcaire, Maria
|e verfasserin
|4 aut
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| 245 |
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|a 3D Organic Nanofabrics
|b Plasma-Assisted Synthesis and Antifreezing Behavior of Superhydrophobic and Lubricant-Infused Slippery Surfaces
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|c 2019
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 04.03.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a Herein, we present the development of supported organic nanofabrics formed by a conformal polymer-like interconnection of small-molecule organic nanowires and nanotrees. These organic nanostructures are fabricated by a combination of vacuum and plasma-assisted deposition techniques to generate step by step, single-crystalline organic nanowires forming one-dimensional building blocks, organic nanotrees applied as three-dimensional templates, and the polymer-like shell that produces the final fabric. The complete procedure is carried out at low temperatures and is compatible with an ample variety of substrates (polymers, metal, ceramics; either planar or in the form of meshes) yielding flexible and low solid-fraction three-dimensional nanostructures. The systematic investigation of this progressively complex organic nanomaterial delivers key clues relating their wetting, nonwetting, and anti-icing properties with their specific morphology and outer surface composition. Water contact angles higher than 150° are attainable as a function of the nanofabric shell thickness with outstanding freezing-delay times (FDT) longer than 2 h at -5 °C. The role of the extremely low roughness of the shell surface is settled as a critical feature for such an achievement. In addition, the characteristic interconnected microstructure of the nanofabrics is demonstrated as ideal for the fabrication of slippery liquid-infused porous surfaces (SLIPS). We present the straightforward deposition of the nanofabric on laser patterns and the knowledge of how this approach provides SLIPS with FDTs longer than 5 h at -5 °C and 1 h at -15 °C
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|a Journal Article
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|a Lopez-Santos, Carmen
|e verfasserin
|4 aut
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|a Aparicio, Francisco J
|e verfasserin
|4 aut
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|a Sanchez-Valencia, Juan R
|e verfasserin
|4 aut
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|a Obrero, Jose M
|e verfasserin
|4 aut
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|a Saghi, Zineb
|e verfasserin
|4 aut
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|a Rico, Victor J
|e verfasserin
|4 aut
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|a de la Fuente, German
|e verfasserin
|4 aut
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|a Gonzalez-Elipe, Agustin R
|e verfasserin
|4 aut
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| 700 |
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|a Barranco, Angel
|e verfasserin
|4 aut
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| 700 |
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|a Borras, Ana
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1992
|g 35(2019), 51 vom: 24. Dez., Seite 16876-16885
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnns
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| 773 |
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|g volume:35
|g year:2019
|g number:51
|g day:24
|g month:12
|g pages:16876-16885
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|u http://dx.doi.org/10.1021/acs.langmuir.9b03116
|3 Volltext
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