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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201905744
|2 doi
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|a pubmed24n1010.xml
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|a (DE-627)NLM303066911
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|a DE-627
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|e rakwb
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|a eng
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|a Wang, Qingyong
|e verfasserin
|4 aut
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|a Redox Tuning in Crystalline and Electronic Structure of Bimetal-Organic Frameworks Derived Cobalt/Nickel Boride/Sulfide for Boosted Faradaic Capacitance
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|c 2019
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 18.12.2019
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a The development of efficient electrode materials is a cutting-edge approach for high-performance energy storage devices. Herein, an effective chemical redox approach is reported for tuning the crystalline and electronic structures of bimetallic cobalt/nickel-organic frameworks (Co-Ni MOFs) to boost faradaic redox reaction for high energy density. The as-obtained cobalt/nickel boride/sulfide exhibits a high specific capacitance (1281 F g-1 at 1 A g-1 ), remarkable rate performance (802.9 F g-1 at 20 A g-1 ), and outstanding cycling stability (92.1% retention after 10 000 cycles). An energy storage device fabricated with a cobalt/nickel boride/sulfide electrode exhibits a high energy density of 50.0 Wh kg-1 at a power density of 857.7 W kg-1 , and capacity retention of 87.7% (up to 5000 cycles at 12 A g-1 ). Such an effective redox approach realizes the systematic electronic tuning that activates the fast faradaic reactions of the metal species in cobalt/nickel boride/sulfide which may shed substantial light on inspiring MOFs and their derivatives for energy storage devices
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|a Journal Article
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|a electronic tuning
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|a energy storage
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|a faradaic capacitance
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|a metal-organic frameworks
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|a redox strategies
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| 700 |
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|a Luo, Yumei
|e verfasserin
|4 aut
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|a Hou, Ruizuo
|e verfasserin
|4 aut
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|a Zaman, Shahid
|e verfasserin
|4 aut
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|a Qi, Kai
|e verfasserin
|4 aut
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| 700 |
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|a Liu, Hongfang
|e verfasserin
|4 aut
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|a Park, Ho Seok
|e verfasserin
|4 aut
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| 700 |
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|a Xia, Bao Yu
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 31(2019), 51 vom: 13. Dez., Seite e1905744
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:31
|g year:2019
|g number:51
|g day:13
|g month:12
|g pages:e1905744
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|u http://dx.doi.org/10.1002/adma.201905744
|3 Volltext
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