Hot-Pressed CsPbBr3 Quasi-Monocrystalline Film for Sensitive Direct X-ray Detection

© 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 31(2019), 44 vom: 13. Nov., Seite e1904405
1. Verfasser: Pan, Weicheng (VerfasserIn)
Weitere Verfasser: Yang, Bo, Niu, Guangda, Xue, Kan-Hao, Du, Xinyuan, Yin, Lixiao, Zhang, Muyi, Wu, Haodi, Miao, Xiang-Shui, Tang, Jiang
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article CsPbBr3 thick films X-ray detectors high sensitivity hot-pressing method
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520 |a An X-ray detector with high sensitivity would be able to increase the generated signal and reduce the dose rate; thus, this type of detector is beneficial for applications such as medical imaging and product inspection. The inorganic lead halide perovskite CsPbBr3 possesses relatively larger density and a higher atomic number in contrast to its hybrid counterpart. Therefore, it is expected to provide high detection sensitivity for X-rays; however, it has rarely been studied as a direct X-ray detector. Here, a hot-pressing method is employed to fabricate thick quasi-monocrystalline CsPbBr3 films, and a record sensitivity of 55 684 µC Gyair -1 cm-2 is achieved, surpassing all other X-ray detectors (direct and indirect). The hot-pressing method is simple and produces thick quasi-monocrystalline CsPbBr3 films with uniform orientations. The high crystalline quality of the CsPbBr3 films and the formation of self-formed shallow bromide vacancy defects during the high-temperature process result in a large µτ product and, therefore, a high photoconductivity gain factor and high detection sensitivity. The detectors also exhibit relatively fast response speed, negligible baseline drift, and good stability, making a CsPbBr3 X-ray detector extremely competitive for high-contrast X-ray detections 
650 4 |a Journal Article 
650 4 |a CsPbBr3 thick films 
650 4 |a X-ray detectors 
650 4 |a high sensitivity 
650 4 |a hot-pressing method 
700 1 |a Yang, Bo  |e verfasserin  |4 aut 
700 1 |a Niu, Guangda  |e verfasserin  |4 aut 
700 1 |a Xue, Kan-Hao  |e verfasserin  |4 aut 
700 1 |a Du, Xinyuan  |e verfasserin  |4 aut 
700 1 |a Yin, Lixiao  |e verfasserin  |4 aut 
700 1 |a Zhang, Muyi  |e verfasserin  |4 aut 
700 1 |a Wu, Haodi  |e verfasserin  |4 aut 
700 1 |a Miao, Xiang-Shui  |e verfasserin  |4 aut 
700 1 |a Tang, Jiang  |e verfasserin  |4 aut 
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773 1 8 |g volume:31  |g year:2019  |g number:44  |g day:13  |g month:11  |g pages:e1904405 
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