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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201903125
|2 doi
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|a eng
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|a Hou, Bao-Hua
|e verfasserin
|4 aut
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|a Self-Supporting, Flexible, Additive-Free, and Scalable Hard Carbon Paper Self-Interwoven by 1D Microbelts
|b Superb Room/Low-Temperature Sodium Storage and Working Mechanism
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|c 2019
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|a Text
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|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Completed 04.10.2019
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Hard carbon is regarded as a promising anode material for sodium-ion batteries (SIBs). However, it usually suffers from the issues of low initial Coulombic efficiency (ICE) and poor rate performance, severely hindering its practical application. Herein, a flexible, self-supporting, and scalable hard carbon paper (HCP) derived from scalable and renewable tissue is rationally designed and prepared as practical additive-free anode for room/low-temperature SIBs with high ICE. In ether electrolyte, such HCP achieves an ICE of up to 91.2% with superior high-rate capability, ultralong cycle life (e.g., 93% capacity retention over 1000 cycles at 200 mA g-1 ) and outstanding low-temperature performance. Working mechanism analyses reveal that the plateau region is the rate-determining step for HCP with a lower electrochemical reaction kinetics, which can be significantly improved in ether electrolyte
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|a Journal Article
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|a anode materials
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|a carbon paper
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|a flexible
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|a sodium-ion batteries
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|a tissue
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|a Wang, Ying-Ying
|e verfasserin
|4 aut
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|a Ning, Qiu-Li
|e verfasserin
|4 aut
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|a Li, Wen-Hao
|e verfasserin
|4 aut
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|a Xi, Xiao-Tong
|e verfasserin
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|a Yang, Xu
|e verfasserin
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|a Liang, Hao-Jie
|e verfasserin
|4 aut
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|a Feng, Xi
|e verfasserin
|4 aut
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|a Wu, Xing-Long
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 31(2019), 40 vom: 11. Okt., Seite e1903125
|w (DE-627)NLM098206397
|x 1521-4095
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|g volume:31
|g year:2019
|g number:40
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|g month:10
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|u http://dx.doi.org/10.1002/adma.201903125
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