|
|
|
|
| LEADER |
01000naa a22002652 4500 |
| 001 |
NLM300130821 |
| 003 |
DE-627 |
| 005 |
20231225101844.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231225s2019 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.201903239
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1000.xml
|
| 035 |
|
|
|a (DE-627)NLM300130821
|
| 035 |
|
|
|a (NLM)31402528
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Zheng, Ding
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Simultaneous Bottom-Up Interfacial and Bulk Defect Passivation in Highly Efficient Planar Perovskite Solar Cells using Nonconjugated Small-Molecule Electrolytes
|
| 264 |
|
1 |
|c 2019
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Completed 04.10.2019
|
| 500 |
|
|
|a Date Revised 01.10.2020
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
|
| 520 |
|
|
|a Recent perovskite solar cell (PSC) advances have pursued strategies for reducing interfacial energetic mismatches to mitigate energy losses, as well as to minimize interfacial and bulk defects and ion vacancies to maximize charge transfer. Here nonconjugated multi-zwitterionic small-molecule electrolytes (NSEs) are introduced, which act not only as charge-extracting layers for barrier-free charge collection at planar triple cation PSC cathodes but also passivate charged defects at the perovskite bulk/interface via a spontaneous bottom-up passivation effect. Implementing these synergistic properties affords NSE-based planar PSCs that deliver a remarkable power conversion efficiency of 21.18% with a maximum VOC = 1.19 V, in combination with suppressed hysteresis and enhanced environmental, thermal, and light-soaking stability. Thus, this work demonstrates that the bottom-up, simultaneous interfacial and bulk trap passivation using NSE modifiers is a promising strategy to overcome outstanding issues impeding further PSC advances
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a bottom-up passivation
|
| 650 |
|
4 |
|a electron-transport layer
|
| 650 |
|
4 |
|a perovskite solar cells
|
| 650 |
|
4 |
|a zwitterions
|
| 700 |
1 |
|
|a Peng, Ruixiang
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Wang, Gang
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Logsdon, Jenna Leigh
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Wang, Binghao
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Hu, Xiaobing
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Chen, Yao
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Dravid, Vinayak P
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Wasielewski, Michael R
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Yu, Junsheng
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Huang, Wei
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Ge, Ziyi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Marks, Tobin J
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Facchetti, Antonio
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 31(2019), 40 vom: 11. Okt., Seite e1903239
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:31
|g year:2019
|g number:40
|g day:11
|g month:10
|g pages:e1903239
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.201903239
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 31
|j 2019
|e 40
|b 11
|c 10
|h e1903239
|