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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201901437
|2 doi
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|a pubmed24n0996.xml
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|a DE-627
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|e rakwb
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|a eng
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| 100 |
1 |
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|a Fu, Beibei
|e verfasserin
|4 aut
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| 245 |
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|a A "Phase Separation" Molecular Design Strategy Towards Large-Area 2D Molecular Crystals
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|c 2019
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a 2D molecular crystals (2DMCs) have attracted considerable attention because of their unique optoelectronic properties and potential applications. Taking advantage of the solution processability of organic semiconductors, solution self-assembly is considered an effective way to grow large-area 2DMCs. However, this route is largely blocked because a precise molecular design towards 2DMCs is missing and little is known about the relationship between 2D solution self-assembly and molecular structure. A "phase separation" molecular design strategy towards 2DMCs is proposed and layer-by-layer growth of millimeter-sized monolayer or few-layer 2DMCs is realized. High-performance organic phototransistors are constructed based on the 2DMCs with unprecedented photosensitivity (2.58 × 107 ), high responsivity (1.91 × 104 A W-1 ), and high detectivity (4.93 × 1015 Jones). This "phase separation" molecular design strategy provides a guide for the design and synthesis of novel organic semiconductors that self-assemble into large-area 2DMCs for advanced organic (opto)electronics
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|a Journal Article
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|a 2D molecular crystals
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|a organic field-effect transistors
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|a organic phototransistors
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|a organic single crystals
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|a phase separation
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|a Wang, Cong
|e verfasserin
|4 aut
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|a Sun, Yantao
|e verfasserin
|4 aut
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|a Yao, Jiarong
|e verfasserin
|4 aut
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|a Wang, Yu
|e verfasserin
|4 aut
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|a Ge, Fayuan
|e verfasserin
|4 aut
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|a Yang, Fangxu
|e verfasserin
|4 aut
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| 700 |
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|a Liu, Zheyuan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Dang, Yanfeng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhang, Xiaotao
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Shao, Xiangfeng
|e verfasserin
|4 aut
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| 700 |
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|a Li, Rongjin
|e verfasserin
|4 aut
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| 700 |
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|a Hu, Wenping
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 31(2019), 35 vom: 01. Aug., Seite e1901437
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:31
|g year:2019
|g number:35
|g day:01
|g month:08
|g pages:e1901437
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|u http://dx.doi.org/10.1002/adma.201901437
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