Diffusion-Freezing-Induced Microphase Separation for Constructing Large-Area Multiscale Structures on Hydrogel Surfaces

© 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 31(2019), 32 vom: 17. Aug., Seite e1808217
1. Verfasser: Lei, Wenwei (VerfasserIn)
Weitere Verfasser: Qi, Shuanhu, Rong, Qinfeng, Huang, Jin, Xu, Yichao, Fang, Ruochen, Liu, Kesong, Jiang, Lei, Liu, Mingjie
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article anti-dehydration hydrogels liquid transport microphase separation multiscale structured surfaces
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520 |a Hydrogels with multiscale structured surface have attracted significant attention for their valuable applications in diverse areas. However, current strategies for the design and fabrication of structured hydrogel surfaces, which suffer from complicated manufacturing processes and specific material modeling, are not efficient to produce structured hydrogel surfaces in large area, and therefore restrict their practical applications. To address this problem, a general and reliable method is reported, which relies on the interplay between polymer chain diffusion and the subsequent freezing-induced gelation and microphase separation processes. The basic idea is systematically analyzed and further exploited to manufacture gel surfaces with gradient structures and patterns through the introduction of temperature gradient and shape control of the contact area. Moreover, the formed micro/nanostructured surfaces are exemplified to work as capillary systems and thus can uplift the liquid spontaneously indicating the potential application for anti-dehydration. It is believed that the proposed facile and large-area fabrication method can inspire the design of materials with various functionalized surfaces 
650 4 |a Journal Article 
650 4 |a anti-dehydration 
650 4 |a hydrogels 
650 4 |a liquid transport 
650 4 |a microphase separation 
650 4 |a multiscale structured surfaces 
700 1 |a Qi, Shuanhu  |e verfasserin  |4 aut 
700 1 |a Rong, Qinfeng  |e verfasserin  |4 aut 
700 1 |a Huang, Jin  |e verfasserin  |4 aut 
700 1 |a Xu, Yichao  |e verfasserin  |4 aut 
700 1 |a Fang, Ruochen  |e verfasserin  |4 aut 
700 1 |a Liu, Kesong  |e verfasserin  |4 aut 
700 1 |a Jiang, Lei  |e verfasserin  |4 aut 
700 1 |a Liu, Mingjie  |e verfasserin  |4 aut 
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