Fate and migration of arsenic in large-scale anaerobic landfill

Copyright © 2019 Elsevier Ltd. All rights reserved.

Bibliographische Detailangaben
Veröffentlicht in:Waste management (New York, N.Y.). - 1999. - 87(2019) vom: 15. März, Seite 559-564
1. Verfasser: Hu, Lifang (VerfasserIn)
Weitere Verfasser: Wang, Wenjie, Long, Yuyang, Wei, Fang, Nie, Zhiyuan, Fang, Chengran
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Waste management (New York, N.Y.)
Schlagworte:Journal Article Anaerobic landfill Arsenic Canonical correlation analysis Sequential extraction procedure Soil Pollutants Iron E1UOL152H7 N712M78A8G
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520 |a The fate and migration of arsenic in a large-scale anaerobic landfill site was investigated by characterization of the total As content and its speciation using a sequential extraction procedure. The total As content in the anaerobic landfill varied greatly with age of the deposited refuse, ranging from 15.26 ± 4.18 mg kg-1 to 38.41 ± 10.41 mg kg-1. There was an increasing trend from the upper layer to a depth of 18-19 m, followed by a decrease in the lower layer. Sequential extraction results showed that As present in exchangeable and weak-acid soluble forms (F1) varied from 0.08 ± 0.01 mg kg-1 to 12.61 ± 0.92 mg kg-1, but from 1.28 ± 0.11 mg kg-1 to 8.40 ± 0.23 mg kg-1 in reducible forms (F2). Oxidizable (F3) and residual (F4) forms of As, which were much more stable and for which the environmental risk correspondingly decreased, accounted for 24.21%-58.70% and 10.11%-30.90% of the total As content, respectively. Nitrate and carbonate had a strong influence on the distribution of As in F1 species; ferric ion affected As distribution in F2; both ferrous ion and dissolved oxygen content contributed to F3 distribution; As in F4 was associated with crystalline minerals structures and was only weakly affected by environmental factors. The deposition process could be divided into six phases to interpret As migration and distribution within the anaerobic landfill after closure 
650 4 |a Journal Article 
650 4 |a Anaerobic landfill 
650 4 |a Arsenic 
650 4 |a Canonical correlation analysis 
650 4 |a Sequential extraction procedure 
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650 7 |a Iron  |2 NLM 
650 7 |a E1UOL152H7  |2 NLM 
650 7 |a Arsenic  |2 NLM 
650 7 |a N712M78A8G  |2 NLM 
700 1 |a Wang, Wenjie  |e verfasserin  |4 aut 
700 1 |a Long, Yuyang  |e verfasserin  |4 aut 
700 1 |a Wei, Fang  |e verfasserin  |4 aut 
700 1 |a Nie, Zhiyuan  |e verfasserin  |4 aut 
700 1 |a Fang, Chengran  |e verfasserin  |4 aut 
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773 1 8 |g volume:87  |g year:2019  |g day:15  |g month:03  |g pages:559-564 
856 4 0 |u http://dx.doi.org/10.1016/j.wasman.2019.02.046  |3 Volltext 
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