Predictive Framework for the Spreading of Liquid Drops and the Formation of Liquid Marbles on Hydrophobic Particle Bed

In this work, we have developed a model to describe the behavior of liquid drops upon impaction on hydrophobic particle bed and verified it experimentally. Poly(tetrafluoroethylene) (PTFE) particles were used to coat drops of water, aqueous solutions of glycerol (20, 40, and 60% v/v), and ethanol (5...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 35(2019), 20 vom: 21. Mai, Seite 6657-6668
1. Verfasser: Mozhi Devan Padmanathan, Arul (VerfasserIn)
Weitere Verfasser: Sneha Ravi, Apoorva, Choudhary, Hema, Varanakkottu, Subramanyan Namboodiri, Dalvi, Sameer V
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article
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100 1 |a Mozhi Devan Padmanathan, Arul  |e verfasserin  |4 aut 
245 1 0 |a Predictive Framework for the Spreading of Liquid Drops and the Formation of Liquid Marbles on Hydrophobic Particle Bed 
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520 |a In this work, we have developed a model to describe the behavior of liquid drops upon impaction on hydrophobic particle bed and verified it experimentally. Poly(tetrafluoroethylene) (PTFE) particles were used to coat drops of water, aqueous solutions of glycerol (20, 40, and 60% v/v), and ethanol (5 and 12% v/v). The experiments were conducted for Weber number ( We) ranging from 8 to 130 and Reynolds number ( Re) ranging from 370 to 4460. The bed porosity was varied from 0.8 to 0.6. The experimental values of βmax (ratio of the diameter at the maximum spreading condition to the initial drop diameter) were estimated from the time-lapsed images captured using a high-speed camera. The theoretical βmax was estimated by making energy balances on the liquid drop. The proposed model accounts for the energy losses due to viscous dissipation and crater formation along with a change in kinetic energy and surface energy. A good agreement was obtained between the experimental βmax and the estimated theoretical βmax. The proposed model yielded a least % absolute average relative deviation (% AARD) of 5.5 ± 4.3 compared to other models available in the literature. Further, it was found that the liquid drops impacting on particle bed are completely coated with PTFE particles with βmax values greater than 2 
650 4 |a Journal Article 
700 1 |a Sneha Ravi, Apoorva  |e verfasserin  |4 aut 
700 1 |a Choudhary, Hema  |e verfasserin  |4 aut 
700 1 |a Varanakkottu, Subramanyan Namboodiri  |e verfasserin  |4 aut 
700 1 |a Dalvi, Sameer V  |e verfasserin  |4 aut 
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