One-Step Preparation Method of Flexible Metafilms on the Water-Oil Interface : Self-Assembly Surface Plasmon Structures for Surface-Enhanced Raman Scattering Detection

The present study demonstrated a one-step method for the first time to fabricate self-assembled gold nanoparticle (AuNP) metafilms at the water-toluene interface by adding polystyrene-polyisoprene-polystyrene as the support layer. The thiolated polyethylene glycol and ethanol were used to tune the s...

Ausführliche Beschreibung

Bibliographische Detailangaben
Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 35(2019), 13 vom: 02. Apr., Seite 4626-4633
1. Verfasser: Yang, Nan (VerfasserIn)
Weitere Verfasser: You, Tingting, Gao, Yukun, Lu, Sichen, Yin, Penggang
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article
LEADER 01000naa a22002652 4500
001 NLM29514856X
003 DE-627
005 20231225083026.0
007 cr uuu---uuuuu
008 231225s2019 xx |||||o 00| ||eng c
024 7 |a 10.1021/acs.langmuir.8b04271  |2 doi 
028 5 2 |a pubmed24n0983.xml 
035 |a (DE-627)NLM29514856X 
035 |a (NLM)30892046 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Yang, Nan  |e verfasserin  |4 aut 
245 1 0 |a One-Step Preparation Method of Flexible Metafilms on the Water-Oil Interface  |b Self-Assembly Surface Plasmon Structures for Surface-Enhanced Raman Scattering Detection 
264 1 |c 2019 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Revised 20.11.2019 
500 |a published: Print-Electronic 
500 |a Citation Status PubMed-not-MEDLINE 
520 |a The present study demonstrated a one-step method for the first time to fabricate self-assembled gold nanoparticle (AuNP) metafilms at the water-toluene interface by adding polystyrene-polyisoprene-polystyrene as the support layer. The thiolated polyethylene glycol and ethanol were used to tune the surface charge density on the AuNPs, constructing a balanced situation at the water-toluene interface. The flexible (AuNP) metafilm can be easily obtained after evaporation of the toluene phase and further used as a surface-enhanced Raman scattering (SERS) substrate for trace thiram detection. The SERS sensitivity was tested using standard Raman probes such as crystal violet and malachite green, both with the detect concentration reaching 1 × 10-11 M. Moreover, the excellent reproducibility and elastic properties make the metafilm promising in practical detection. Hence, the trace thiram detection on an orange pericarp was inspected with the detection limit of 0.5 ppm (1 × 10-6 M) as well as a favorable linearity relation with a correlation coefficient of 0.979, exactly matching the realistic application requirements 
650 4 |a Journal Article 
700 1 |a You, Tingting  |e verfasserin  |4 aut 
700 1 |a Gao, Yukun  |e verfasserin  |4 aut 
700 1 |a Lu, Sichen  |e verfasserin  |4 aut 
700 1 |a Yin, Penggang  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Langmuir : the ACS journal of surfaces and colloids  |d 1992  |g 35(2019), 13 vom: 02. Apr., Seite 4626-4633  |w (DE-627)NLM098181009  |x 1520-5827  |7 nnns 
773 1 8 |g volume:35  |g year:2019  |g number:13  |g day:02  |g month:04  |g pages:4626-4633 
856 4 0 |u http://dx.doi.org/10.1021/acs.langmuir.8b04271  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_22 
912 |a GBV_ILN_350 
912 |a GBV_ILN_721 
951 |a AR 
952 |d 35  |j 2019  |e 13  |b 02  |c 04  |h 4626-4633