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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201807577
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|a pubmed24n0983.xml
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|a (DE-627)NLM295068787
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|a (NLM)30883937
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Yuan, Jun
|e verfasserin
|4 aut
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|a Fused Benzothiadiazole
|b A Building Block for n-Type Organic Acceptor to Achieve High-Performance Organic Solar Cells
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|c 2019
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Narrow bandgap n-type organic semiconductors (n-OS) have attracted great attention in recent years as acceptors in organic solar cells (OSCs), due to their easily tuned absorption and electronic energy levels in comparison with fullerene acceptors. Herein, a new n-OS acceptor, Y5, with an electron-deficient-core-based fused structure is designed and synthesized, which exhibits a strong absorption in the 600-900 nm region with an extinction coefficient of 1.24 × 105 cm-1 , and an electron mobility of 2.11 × 10-4 cm2 V-1 s-1 . By blending Y5 with three types of common medium-bandgap polymers (J61, PBDB-T, and TTFQx-T1) as donors, all devices exhibit high short-circuit current densities over 20 mA cm-2 . As a result, the power conversion efficiency of the Y5-based OSCs with J61, TTFQx-T1, and PBDB-T reaches 11.0%, 13.1%, and 14.1%, respectively. This indicates that Y5 is a universal and highly efficient n-OS acceptor for applications in organic solar cells
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|a Journal Article
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|a electron-deficient core
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|a fused benzothiadiazole
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|a nonfullerene acceptors
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|a organic photovoltaics
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|a power conversion efficiency
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|a Zhang, Yunqiang
|e verfasserin
|4 aut
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|a Zhou, Liuyang
|e verfasserin
|4 aut
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|a Zhang, Chujun
|e verfasserin
|4 aut
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|a Lau, Tsz-Ki
|e verfasserin
|4 aut
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|a Zhang, Guichuan
|e verfasserin
|4 aut
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|a Lu, Xinhui
|e verfasserin
|4 aut
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|a Yip, Hin-Lap
|e verfasserin
|4 aut
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|a So, Shu Kong
|e verfasserin
|4 aut
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|a Beaupré, Serge
|e verfasserin
|4 aut
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|a Mainville, Mathieu
|e verfasserin
|4 aut
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|a Johnson, Paul A
|e verfasserin
|4 aut
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|a Leclerc, Mario
|e verfasserin
|4 aut
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|a Chen, Honggang
|e verfasserin
|4 aut
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|a Peng, Hongjian
|e verfasserin
|4 aut
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|a Li, Yongfang
|e verfasserin
|4 aut
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|a Zou, Yingping
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 31(2019), 17 vom: 07. Apr., Seite e1807577
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:31
|g year:2019
|g number:17
|g day:07
|g month:04
|g pages:e1807577
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|u http://dx.doi.org/10.1002/adma.201807577
|3 Volltext
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