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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.8b03849
|2 doi
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|a pubmed24n0977.xml
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|a (NLM)30702296
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Armstrong, Steven
|e verfasserin
|4 aut
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|a Pinning-Free Evaporation of Sessile Droplets of Water from Solid Surfaces
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|c 2019
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 20.11.2019
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a Contact-line pinning is a fundamental limitation to the motion of contact lines of liquids on solid surfaces. When a sessile droplet evaporates, contact-line pinning typically results in either a stick-slip evaporation mode, where the contact line pins and depins from the surface in an uncontrolled manner, or a constant contact-area mode with a pinned contact line. Pinning prevents the observation of the quasi-equilibrium constant contact-angle mode of evaporation, which has never been observed for sessile droplets of water directly resting on a smooth, nontextured, solid surface. Here, we report the evaporation of a sessile droplet from a flat glass substrate treated with a smooth, slippery, omni-phobic covalently attached liquid-like coating. Our characterization of the surfaces shows high contact line mobility with an extremely low contact-angle hysteresis of ∼1° and reveals a step change in the value of the contact angle from 101° to 105° between a relative humidity (RH) of 30 and 40%, in a manner reminiscent of the transition observed in a type V adsorption isotherm. We observe the evaporation of small sessile droplets in a chamber held at a constant temperature, T = (25.0 ± 0.1) °C and at constant RH across the range RH = 10-70%. In all cases, a constant contact-angle mode of evaporation is observed for most of the evaporation time. Furthermore, we analyze the evaporation sequences using the Picknett and Bexon ideal constant contact-angle mode for diffusion-limited evaporation. The resulting estimate for the diffusion coefficient, DE, of water vapor in air of DE = (2.44 ± 0.48) × 10-5 m2 s-1 is accurate to within 2% of the value reported in the literature, thus validating the constant contact-angle mode of the diffusion-limited evaporation model
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|a Journal Article
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|a McHale, Glen
|e verfasserin
|4 aut
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|a Ledesma-Aguilar, Rodrigo
|e verfasserin
|4 aut
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|a Wells, Gary G
|e verfasserin
|4 aut
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1992
|g 35(2019), 8 vom: 26. Feb., Seite 2989-2996
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnns
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|g volume:35
|g year:2019
|g number:8
|g day:26
|g month:02
|g pages:2989-2996
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|u http://dx.doi.org/10.1021/acs.langmuir.8b03849
|3 Volltext
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|d 35
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