Chemical Approaches to Carbon-Based Metal-Free Catalysts

Chemical Approaches to Carbon-Based Metal-Free Catalysts

© 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 31(2019), 13 vom: 10. März, Seite e1804863
1. Verfasser: Liu, Dong (VerfasserIn)
Weitere Verfasser: Dai, Liming, Lin, Xuanni, Chen, Jian-Feng, Zhang, Jian, Feng, Xinliang, Müllen, Klaus, Zhu, Xiang, Dai, Sheng
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article Review carbon chemical approaches electrocatalysts metal-free catalysts photocatalysts
Beschreibung
Zusammenfassung:© 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Highly active and durable catalysts play a key role in clean energy technologies. However, the high cost, low reserves, and poor stability of noble-metal-based catalysts have hindered the large-scale development of renewable energy. Owing to their low cost, earth abundance, high activity, and excellent stability, carbon-based metal-free catalysts (CMFCs) are promising alternatives to precious-metal-based catalysts. Although many synthetic methods based on solution, surface/interface, solid state, and noncovalent chemistries have been developed for producing numerous CMFCs with diverse structures and functionalities, there is still a lack of effective approaches to precisely control the structures of active sites. Therefore, novel chemical approaches are needed for the development of highly active and durable CMFCs that are capable of replacing precious-metal catalysts for large-scale applications. Herein, a comprehensive and critical review on chemical approaches to CMFCs is given by summarizing important advancements, current challenges, and future perspectives in this emerging field. Through such a critical review, our understanding of CMFCs and the associated synthetic processes will be significantly increased
Beschreibung:Date Completed 26.03.2019
Date Revised 01.10.2020
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1521-4095
DOI:10.1002/adma.201804863