Multifunctional "Hydrogel Skins" on Diverse Polymers with Arbitrary Shapes

© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 31(2019), 7 vom: 20. Feb., Seite e1807101
1. Verfasser: Yu, Yan (VerfasserIn)
Weitere Verfasser: Yuk, Hyunwoo, Parada, German A, Wu, You, Liu, Xinyue, Nabzdyk, Christoph S, Youcef-Toumi, Kamal, Zang, Jianfeng, Zhao, Xuanhe
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article antifouling biomedical devices coatings hydrogels low friction polymer devices
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520 |a Slippery and hydrophilic surfaces find critical applications in areas as diverse as biomedical devices, microfluidics, antifouling, and underwater robots. Existing methods to achieve such surfaces rely mostly on grafting hydrophilic polymer brushes or coating hydrogel layers, but these methods suffer from several limitations. Grafted polymer brushes are prone to damage and do not provide sufficient mechanical compliance due to their nanometer-scale thickness. Hydrogel coatings are applicable only for relatively simple geometries, precluding their use for the surfaces with complex geometries and features. Here, a new method is proposed to interpenetrate hydrophilic polymers into the surface of diverse polymers with arbitrary shapes to form naturally integrated "hydrogel skins." The hydrogel skins exhibit tissue-like softness (Young's modulus ≈ 30 kPa), have uniform and tunable thickness in the range of 5-25 µm, and can withstand prolonged shearing forces with no measurable damage. The hydrogel skins also provide superior low-friction, antifouling, and ionically conductive surfaces to the polymer substrates without compromising their original mechanical properties and geometry. Applications of the hydrogel skins on inner and outer surfaces of various practical polymer devices including medical tubing, Foley catheters, cardiac pacemaker leads, and soft robots on massive scales are further demonstrated 
650 4 |a Journal Article 
650 4 |a antifouling 
650 4 |a biomedical devices 
650 4 |a coatings 
650 4 |a hydrogels 
650 4 |a low friction 
650 4 |a polymer devices 
700 1 |a Yuk, Hyunwoo  |e verfasserin  |4 aut 
700 1 |a Parada, German A  |e verfasserin  |4 aut 
700 1 |a Wu, You  |e verfasserin  |4 aut 
700 1 |a Liu, Xinyue  |e verfasserin  |4 aut 
700 1 |a Nabzdyk, Christoph S  |e verfasserin  |4 aut 
700 1 |a Youcef-Toumi, Kamal  |e verfasserin  |4 aut 
700 1 |a Zang, Jianfeng  |e verfasserin  |4 aut 
700 1 |a Zhao, Xuanhe  |e verfasserin  |4 aut 
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773 1 8 |g volume:31  |g year:2019  |g number:7  |g day:20  |g month:02  |g pages:e1807101 
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