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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201804883
|2 doi
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|a pubmed25n0972.xml
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|a eng
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| 100 |
1 |
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|a Zhang, Huabin
|e verfasserin
|4 aut
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|a Ultrasmall MoOx Clusters as a Novel Cocatalyst for Photocatalytic Hydrogen Evolution
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|c 2019
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|a Text
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|a ƒaComputermedien
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|a Date Completed 11.02.2019
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a To enhance the performance of semiconductor photocatalysts, cocatalysts are used to accelerate surface reactions. Herein, ultrasmall molybdenum-oxygen (MoOx ) clusters are developed as a novel non-noble cocatalyst, which significantly promotes the photocatalytic hydrogen generation rate of CdS nanowires (NWs). As indicated by extended X-ray absorption fine structure analysis, direct bonds are formed between CdS NWs and MoOx clusters, which guarantee the migration of photo-generated charge carriers. Moreover, the MoOx clusters induce deep electron trap states owing to the unique atomic arrangement and configuration with the generation of long-lived electrons to enhance the activity. These findings may guide the design of efficient cocatalytic materials for solar water splitting and open a new avenue toward practical applications of ultrasmall clusters
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|a Journal Article
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|a CdS
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|a MoOx
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|a clusters
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|a hydrogen evolution reaction
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|a nanostructures
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|a Zhang, Peng
|e verfasserin
|4 aut
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|a Qiu, Mei
|e verfasserin
|4 aut
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1 |
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|a Dong, Juncai
|e verfasserin
|4 aut
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|a Zhang, Yongfan
|e verfasserin
|4 aut
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|a Lou, Xiong Wen David
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 31(2019), 6 vom: 15. Feb., Seite e1804883
|w (DE-627)NLM098206397
|x 1521-4095
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|g volume:31
|g year:2019
|g number:6
|g day:15
|g month:02
|g pages:e1804883
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|u http://dx.doi.org/10.1002/adma.201804883
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