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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201805472
|2 doi
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|a pubmed24n0967.xml
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|a (DE-627)NLM290272319
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|a (NLM)30393920
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|a DE-627
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|c DE-627
|e rakwb
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|a eng
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| 100 |
1 |
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|a Persson, Ingemar
|e verfasserin
|4 aut
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|a 2D Transition Metal Carbides (MXenes) for Carbon Capture
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|c 2019
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 11.01.2019
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Global warming caused by burning of fossil fuels is indisputably one of mankind's greatest challenges in the 21st century. To reduce the ever-increasing CO2 emissions released into the atmosphere, dry solid adsorbents with large surface-to-volume ratio such as carbonaceous materials, zeolites, and metal-organic frameworks have emerged as promising material candidates for capturing CO2 . However, challenges remain because of limited CO2 /N2 selectivity and long-term stability. The effective adsorption of CO2 gas (≈12 mol kg-1 ) on individual sheets of 2D transition metal carbides (referred to as MXenes) is reported here. It is shown that exposure to N2 gas results in no adsorption, consistent with first-principles calculations. The adsorption efficiency combined with the CO2 /N2 selectivity, together with a chemical and thermal stability, identifies the archetype Ti3 C2 MXene as a new material for carbon capture (CC) applications
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|a Journal Article
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|a MXene
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|a carbon capture
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|a environmental TEM
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4 |
|a surface terminations
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|a Halim, Joseph
|e verfasserin
|4 aut
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|a Lind, Hans
|e verfasserin
|4 aut
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|a Hansen, Thomas W
|e verfasserin
|4 aut
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|a Wagner, Jakob B
|e verfasserin
|4 aut
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|a Näslund, Lars-Åke
|e verfasserin
|4 aut
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|a Darakchieva, Vanya
|e verfasserin
|4 aut
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|a Palisaitis, Justinas
|e verfasserin
|4 aut
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|a Rosen, Johanna
|e verfasserin
|4 aut
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|a Persson, Per O Å
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 31(2019), 2 vom: 02. Jan., Seite e1805472
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:31
|g year:2019
|g number:2
|g day:02
|g month:01
|g pages:e1805472
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|u http://dx.doi.org/10.1002/adma.201805472
|3 Volltext
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