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231225s2018 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201805175
|2 doi
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|a pubmed25n0964.xml
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|a (DE-627)NLM289379814
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|a (NLM)30302837
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|a DE-627
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|e rakwb
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|a eng
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| 100 |
1 |
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|a Xing, Pengyao
|e verfasserin
|4 aut
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| 245 |
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|a Programmable Multicomponent Self-Assembly Based on Aromatic Amino Acids
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|c 2018
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Completed 22.03.2019
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status MEDLINE
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|a © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Construction of integrated self-assembly with ordered structures from two or more organic building blocks is currently a challenge, since it suffers from intrinsic systematic complexity and diverse competitive pathways. Here, it is reported that aromatic amino acid building units can be incorporated into two- or three-component coassembly driven primarily by hydrogen bonding interactions without the assistance of metal-ligand and macrocycle-based host-guest interactions. The key strategy is to employ a C3 -symmetric molecule with alternative hydrogen bonding donor/acceptor sites that are able to bind either carboxylic acid or pyridine appended building units. Aromatic amino acids, C3 -symmetric compound, and bipyridine unit constitute a unique ternary mutual binding system, where three coassembly pathways including two pairwise formations and one ternary combination are unveiled, giving rise to two- and three-component self-assemblies with ordered structures, respectively. The pathway complexity lies in the structural parameter of aromatic amino acids, which can be programmable by controlling substituents at the α-position of amino acids
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|a Journal Article
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|a aromatic amino acids
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|a hydrogen bonding
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|a multicomponent self-assembly
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|a superchirality
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|a ternary coassembly
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|a Amino Acids, Aromatic
|2 NLM
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|a Carboxylic Acids
|2 NLM
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|a Ligands
|2 NLM
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|a Pyridines
|2 NLM
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|a pyridine
|2 NLM
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| 650 |
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|a NH9L3PP67S
|2 NLM
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| 700 |
1 |
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|a Phua, Soo Zeng Fiona
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wei, Xuan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhao, Yanli
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 30(2018), 49 vom: 15. Dez., Seite e1805175
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:30
|g year:2018
|g number:49
|g day:15
|g month:12
|g pages:e1805175
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|u http://dx.doi.org/10.1002/adma.201805175
|3 Volltext
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