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231225s2018 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201804033
|2 doi
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|a pubmed24n0964.xml
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|a (DE-627)NLM289207649
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|a (NLM)30285284
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|a DE-627
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|a eng
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|a Lu, Haijiao
|e verfasserin
|4 aut
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|a Single-Source Bismuth (Transition Metal) Polyoxovanadate Precursors for the Scalable Synthesis of Doped BiVO4 Photoanodes
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|c 2018
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Completed 13.11.2018
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2018 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Single-source precursors are used to produce nanostructured BiVO4 photoanodes for water oxidation in a straightforward and scalable drop-casting synthetic process. Polyoxometallate precursors, which contain both Bi and V, are produced in a one-step reaction from commercially available starting materials. Simple annealing of the molecular precursor produces nanocrystalline BiVO4 films. The precursor can be designed to incorporate a third metal (Co, Ni, Cu, or Zn), enabling the direct formation of doped BiVO4 films. In particular, the Co- and Zn-doped photoanodes show promise for photoelectrochemical water oxidation, with photocurrent densities >1 mA cm-2 at 1.23 V vs reversible hydrogen electrode (RHE). Using this simple synthetic process, a 300 cm2 Co-BiVO4 photoanode is produced, which generates a photocurrent of up to 67 mA at 1.23 V vs RHE and demonstrates the scalability of this approach
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|a Journal Article
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|a BiVO4
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|a doping
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|a polyoxovanadate
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|a single-source precursor
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|a water oxidation
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|a Andrei, Virgil
|e verfasserin
|4 aut
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|a Jenkinson, Kellie J
|e verfasserin
|4 aut
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|a Regoutz, Anna
|e verfasserin
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|a Li, Ning
|e verfasserin
|4 aut
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|a Creissen, Charles E
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|4 aut
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|a Wheatley, Andrew E H
|e verfasserin
|4 aut
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|a Hao, Hongxun
|e verfasserin
|4 aut
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|a Reisner, Erwin
|e verfasserin
|4 aut
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|a Wright, Dominic S
|e verfasserin
|4 aut
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|a Pike, Sebastian D
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 30(2018), 46 vom: 18. Nov., Seite e1804033
|w (DE-627)NLM098206397
|x 1521-4095
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|g volume:30
|g year:2018
|g number:46
|g day:18
|g month:11
|g pages:e1804033
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