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231225s2018 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.8b02785
|2 doi
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|a pubmed25n0963.xml
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|a eng
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| 100 |
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|a Chen, Zhe
|e verfasserin
|4 aut
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|a Pd Nanoparticles Confined in the Porous Graphene-like Carbon Nanosheets for Olefin Hydrogenation
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|c 2018
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|a Text
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|a ƒaComputermedien
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|a Date Completed 02.01.2019
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|a Date Revised 02.01.2019
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a As a novel type of defective graphene, porous graphene has been considered an excellent support material for metal clusters, as the interaction between defective carbon atoms surrounded with the metal nanoparticles (NPs) is very different from that on the ordinary supported catalyst. In this work, we reported a facile three-step method to confine the Pd NPs and grow the graphene-like carbon nanosheets (GLCs) in the same interlayer space of the layered silicate, generating embedded Pd NPs in the pores of porous GLCs in situ. The PdGLC nanocomposite exhibited not only high activity and stability than the common commercial Pd/C catalyst for the hydrogenation of olefins but also superior ability of resisting high temperature, which benefitted from the two-dimensional structure of layered GLCs, the confinement of Pd, and the increased edge and defect of the unsaturated carbon atoms in GLCs
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|a Journal Article
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|a Research Support, Non-U.S. Gov't
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|a Wang, Weixue
|e verfasserin
|4 aut
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|a Zhang, Yifei
|e verfasserin
|4 aut
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| 700 |
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|a Liang, Yu
|e verfasserin
|4 aut
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|a Cui, Zhimin
|e verfasserin
|4 aut
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|a Wang, Xiangke
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1985
|g 34(2018), 43 vom: 30. Okt., Seite 12809-12814
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|x 1520-5827
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|g volume:34
|g year:2018
|g number:43
|g day:30
|g month:10
|g pages:12809-12814
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|u http://dx.doi.org/10.1021/acs.langmuir.8b02785
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