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231225s2019 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201803762
|2 doi
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|a eng
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| 100 |
1 |
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|a Zuo, Zicheng
|e verfasserin
|4 aut
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|a Synthesis and Applications of Graphdiyne-Based Metal-Free Catalysts
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|c 2019
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|a Text
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Completed 26.03.2019
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a The development of carbon materials offers the hope for obtaining inexpensive and high-performance alternatives to substitute noble-metal catalysts for their sustainable application. Graphdiyne, the rising-star carbon allotrope, is a big family with many members, and first realized the coexistence of sp- and sp2 -hybridized carbon atoms in a 2D planar structure. Different from the prevailing carbon materials, its nonuniform distribution in the electronic structure and wide tunability in bandgap show many possibilities and special inspirations to construct new-concept metal-free catalysts, and provide many opportunities for achieving a catalytic activity comparable with that of noble-metal catalysts. Herein, the recent progress in synthetic methodologies, theoretical predictions, and experimental investigations of graphdiyne for metal-free catalysts is systematically summarized. Some new perspectives of the opportunities and challenges in developing high-performance graphdiyne-based metal-free catalysts are demonstrated
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|a Journal Article
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|a Review
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|a graphdiyne
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|a metal-free catalysts
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|a oxygen reduction reaction
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|a photocatalysts
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|a water splitting
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|a Wang, Dan
|e verfasserin
|4 aut
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|a Zhang, Jin
|e verfasserin
|4 aut
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|a Lu, Fushen
|e verfasserin
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|a Li, Yuliang
|e verfasserin
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|t Advanced materials (Deerfield Beach, Fla.)
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|g 31(2019), 13 vom: 30. März, Seite e1803762
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|g volume:31
|g year:2019
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|g day:30
|g month:03
|g pages:e1803762
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