Combined processes of ozonation and supercritical water oxidation for landfill leachate degradation

Copyright © 2018 Elsevier Ltd. All rights reserved.

Bibliographische Detailangaben
Veröffentlicht in:Waste management (New York, N.Y.). - 1999. - 77(2018) vom: 01. Juli, Seite 466-476
1. Verfasser: Scandelai, Ana Paula Jambers (VerfasserIn)
Weitere Verfasser: Cardozo Filho, Lúcio, Martins, Danielly Cruz Campos, Freitas, Thabata Karoliny Formicoli de Souza, Garcia, Juliana Carla, Tavares, Célia Regina Granhen
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2018
Zugriff auf das übergeordnete Werk:Waste management (New York, N.Y.)
Schlagworte:Journal Article AOP Organic compounds Organic matter Ozone ScWO Supercritical oxidation Water Pollutants, Chemical Water 059QF0KO0R 66H7ZZK23N
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520 |a Leachate is a highly variable, heterogeneous and recalcitrant wastewater generated in landfills which may contain high concentrations of many organic and inorganic compounds, hampering the application of a single technique in its treatment. Therefore, this paper assessed leachate degradation through supercritical water oxidation (ScWO) as well as combined processes of ozonation and supercritical water oxidation (O3/ScWO and ScWO/O3), a yet innovative combination. Ozonation was carried out at different reaction times (30-120 min). ScWO was developed at 600 °C, 23 MPa, and spatial time (τ) from 29 to 52 s. A combination of ozonation (30 min) and supercritical water oxidation process (O3-30'/ScWO) was the most efficient technique for the degradation of the leachate assessed. These conditions enabled to remove high values of apparent and true color (92% and 97%, respectively), biochemical oxygen demand (BOD5,20) (95%), chemical oxygen demand (COD) (92%), total organic carbon (TOC) (79%), nitrite (78%), nitrate (84%), total (96%), dissolved (96%) and suspended (94%) solids. In addition, the combined process presented significant decrease in electric conductivity (EC) (68%) and less leachate turbidity removal (43%). Except for ammonia and nitrite, all parameters of the leachate treated by O3-30'/ScWO met the specifications of Brazilian legislation (CONAMA Resolutions No. 357/2005 and No. 430/2011) for the disposal of wastewater in water bodies. Besides, both processes are considered to be clean technologies. This shows the great possibility of applying the O3/ScWO combination to landfills leachates 
650 4 |a Journal Article 
650 4 |a AOP 
650 4 |a Organic compounds 
650 4 |a Organic matter 
650 4 |a Ozone 
650 4 |a ScWO 
650 4 |a Supercritical oxidation 
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650 7 |a Water  |2 NLM 
650 7 |a 059QF0KO0R  |2 NLM 
650 7 |a Ozone  |2 NLM 
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700 1 |a Cardozo Filho, Lúcio  |e verfasserin  |4 aut 
700 1 |a Martins, Danielly Cruz Campos  |e verfasserin  |4 aut 
700 1 |a Freitas, Thabata Karoliny Formicoli de Souza  |e verfasserin  |4 aut 
700 1 |a Garcia, Juliana Carla  |e verfasserin  |4 aut 
700 1 |a Tavares, Célia Regina Granhen  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Waste management (New York, N.Y.)  |d 1999  |g 77(2018) vom: 01. Juli, Seite 466-476  |w (DE-627)NLM098197061  |x 1879-2456  |7 nnns 
773 1 8 |g volume:77  |g year:2018  |g day:01  |g month:07  |g pages:466-476 
856 4 0 |u http://dx.doi.org/10.1016/j.wasman.2018.04.031  |3 Volltext 
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