3D-Printing Electrolytes for Solid-State Batteries

© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 30(2018), 18 vom: 25. Mai, Seite e1707132
1. Verfasser: McOwen, Dennis W (VerfasserIn)
Weitere Verfasser: Xu, Shaomao, Gong, Yunhui, Wen, Yang, Godbey, Griffin L, Gritton, Jack E, Hamann, Tanner R, Dai, Jiaqi, Hitz, Gregory T, Hu, Liangbing, Wachsman, Eric D
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2018
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article 3D printing additive manufacturing lithium metal solid electrolytes solid-state batteries
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520 |a Solid-state batteries have many enticing advantages in terms of safety and stability, but the solid electrolytes upon which these batteries are based typically lead to high cell resistance. Both components of the resistance (interfacial, due to poor contact with electrolytes, and bulk, due to a thick electrolyte) are a result of the rudimentary manufacturing capabilities that exist for solid-state electrolytes. In general, solid electrolytes are studied as flat pellets with planar interfaces, which minimizes interfacial contact area. Here, multiple ink formulations are developed that enable 3D printing of unique solid electrolyte microstructures with varying properties. These inks are used to 3D-print a variety of patterns, which are then sintered to reveal thin, nonplanar, intricate architectures composed only of Li7 La3 Zr2 O12 solid electrolyte. Using these 3D-printing ink formulations to further study and optimize electrolyte structure could lead to solid-state batteries with dramatically lower full cell resistance and higher energy and power density. In addition, the reported ink compositions could be used as a model recipe for other solid electrolyte or ceramic inks, perhaps enabling 3D printing in related fields 
650 4 |a Journal Article 
650 4 |a 3D printing 
650 4 |a additive manufacturing 
650 4 |a lithium metal 
650 4 |a solid electrolytes 
650 4 |a solid-state batteries 
700 1 |a Xu, Shaomao  |e verfasserin  |4 aut 
700 1 |a Gong, Yunhui  |e verfasserin  |4 aut 
700 1 |a Wen, Yang  |e verfasserin  |4 aut 
700 1 |a Godbey, Griffin L  |e verfasserin  |4 aut 
700 1 |a Gritton, Jack E  |e verfasserin  |4 aut 
700 1 |a Hamann, Tanner R  |e verfasserin  |4 aut 
700 1 |a Dai, Jiaqi  |e verfasserin  |4 aut 
700 1 |a Hitz, Gregory T  |e verfasserin  |4 aut 
700 1 |a Hu, Liangbing  |e verfasserin  |4 aut 
700 1 |a Wachsman, Eric D  |e verfasserin  |4 aut 
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773 1 8 |g volume:30  |g year:2018  |g number:18  |g day:25  |g month:05  |g pages:e1707132 
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