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231225s2018 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201704546
|2 doi
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|a pubmed24n0930.xml
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|a (DE-627)NLM278999522
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|a (NLM)29235212
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Fan, Qunping
|e verfasserin
|4 aut
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|a High-Performance As-Cast Nonfullerene Polymer Solar Cells with Thicker Active Layer and Large Area Exceeding 11% Power Conversion Efficiency
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|c 2018
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 01.08.2018
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a In this work, a nonfullerene polymer solar cell (PSC) based on a wide bandgap polymer donor PM6 containing fluorinated thienyl benzodithiophene (BDT-2F) unit and a narrow bandgap small molecule acceptor 2,2'-((2Z,2'Z)-((4,4,9,9-tetrahexyl-4,9-dihydro-s-indaceno[1,2-b:5,6-b']dithiophene-2,7-diyl)bis(methanylylidene))bis(3-oxo-2,3-dihydro-1H-indene-2,1-diylidene))dimalononitrile (IDIC) is developed. In addition to matched energy levels and complementary absorption spectrum with IDIC, PM6 possesses high crystallinity and strong π-π stacking alignment, which are favorable to charge carrier transport and hence suppress recombination in devices. As a result, the PM6:IDIC-based PSCs without extra treatments show an outstanding power conversion efficiency (PCE) of 11.9%, which is the record value for the as-cast PSC devices reported in the literature to date. Moreover, the device performances are insensitive to the active layer thickness (≈95-255 nm) and device area (0.20-0.81 cm2 ) with PCEs of over 11%. Besides, the PM6:IDIC-based flexible PSCs with a large device area of 1.25 cm2 exhibit a high PCE of 6.54%. These results indicate that the PM6:IDIC blend is a promising candidate for future roll-to-roll mass manufacturing and practical application of highly efficient PSCs
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|a Journal Article
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|a large area
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|a nonfullerene polymer solar cells
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|a thicker active layer
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|a wide-bandgap polymer donor
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|a without extra treatments
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|a Wang, Yan
|e verfasserin
|4 aut
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|a Zhang, Maojie
|e verfasserin
|4 aut
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|a Wu, Bo
|e verfasserin
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|a Guo, Xia
|e verfasserin
|4 aut
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|a Jiang, Yufeng
|e verfasserin
|4 aut
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|a Li, Wanbin
|e verfasserin
|4 aut
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|a Guo, Bing
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|a Ye, Chennan
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|a Su, Wenyan
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|a Fang, Jin
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|a Ou, Xuemei
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|a Liu, Feng
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|a Wei, Zhixiang
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|a Sum, Tze Chien
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|a Russell, Thomas P
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|a Li, Yongfang
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 30(2018), 6 vom: 02. Feb.
|w (DE-627)NLM098206397
|x 1521-4095
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|g volume:30
|g year:2018
|g number:6
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|g month:02
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|u http://dx.doi.org/10.1002/adma.201704546
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