Selective Low-Energy Carbon Dioxide Adsorption Using Monodisperse Nitrogen-Rich Hollow Carbon Submicron Spheres

Selective Low-Energy Carbon Dioxide Adsorption Using Monodisperse Nitrogen-Rich Hollow Carbon Submicron Spheres

Monodisperse, nitrogen-doped hollow carbon spheres of submicron size were synthesized using hexamethoxymethylmelamine as both a carbon and nitrogen source in a short (1 h) microwave-assisted synthesis. After carbonization at 550 °C, porous carbon spheres with a remarkably high nitrogen content of 37...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1999. - 34(2018), 1 vom: 09. Jan., Seite 30-35
1. Verfasser: Arif, Aditya F (VerfasserIn)
Weitere Verfasser: Kobayashi, Yuma, Schneider, Elia M, Hess, Samuel C, Balgis, Ratna, Izawa, Takafumi, Iwasaki, Hideharu, Taniguchi, Shuto, Ogi, Takashi, Okuyama, Kikuo, Stark, Wendelin J
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2018
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Research Support, Non-U.S. Gov't
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520 |a Monodisperse, nitrogen-doped hollow carbon spheres of submicron size were synthesized using hexamethoxymethylmelamine as both a carbon and nitrogen source in a short (1 h) microwave-assisted synthesis. After carbonization at 550 °C, porous carbon spheres with a remarkably high nitrogen content of 37.1% were obtained, which consisting mainly of highly basic pyridinic moieties. The synthesized hollow spheres exhibited high selectivity for carbon dioxide (CO2) over nitrogen and oxygen gases, with a capture capacity up to 1.56 mmol CO2 g-1. The low adsorption enthalpy of the synthesized hollow carbon spheres permits good adsorbent regeneration. Evaluation of the feasibility of scaling up shows their potential for large-scale applications 
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650 4 |a Research Support, Non-U.S. Gov't 
700 1 |a Kobayashi, Yuma  |e verfasserin  |4 aut 
700 1 |a Schneider, Elia M  |e verfasserin  |4 aut 
700 1 |a Hess, Samuel C  |e verfasserin  |4 aut 
700 1 |a Balgis, Ratna  |e verfasserin  |4 aut 
700 1 |a Izawa, Takafumi  |e verfasserin  |4 aut 
700 1 |a Iwasaki, Hideharu  |e verfasserin  |4 aut 
700 1 |a Taniguchi, Shuto  |e verfasserin  |4 aut 
700 1 |a Ogi, Takashi  |e verfasserin  |4 aut 
700 1 |a Okuyama, Kikuo  |e verfasserin  |4 aut 
700 1 |a Stark, Wendelin J  |e verfasserin  |4 aut 
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