Synthesis of Carbon Dots with Multiple Color Emission by Controlled Graphitization and Surface Functionalization

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 30(2018), 1 vom: 05. Jan.
1. Verfasser: Miao, Xiang (VerfasserIn)
Weitere Verfasser: Qu, Dan, Yang, Dongxue, Nie, Bing, Zhao, Yikang, Fan, Hongyou, Sun, Zaicheng
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2018
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article carbon dots effective conjugation length light-emitting devices multiple-color emission phosphors
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520 |a Multiple-color-emissive carbon dots (CDots) have potential applications in various fields such as bioimaging, light-emitting devices, and photocatalysis. The majority of the current CDots to date exhibit excitation-wavelength-dependent emissions with their maximum emission limited at the blue-light region. Here, a synthesis of multiple-color-emission CDots by controlled graphitization and surface function is reported. The CDots are synthesized through controlled thermal pyrolysis of citric acid and urea. By regulating the thermal-pyrolysis temperature and ratio of reactants, the maximum emission of the resulting CDots gradually shifts from blue to red light, covering the entire light spectrum. Specifically, the emission position of the CDots can be tuned from 430 to 630 nm through controlling the extent of graphitization and the amount of surface functional groups, COOH. The relative photoluminescence quantum yields of the CDots with blue, green, and red emission reach up to 52.6%, 35.1%, and 12.9%, respectively. Furthermore, it is demonstrated that the CDots can be uniformly dispersed into epoxy resins and be fabricated as transparent CDots/epoxy composites for multiple-color- and white-light-emitting devices. This research opens a door for developing low-cost CDots as alternative phosphors for light-emitting devices 
650 4 |a Journal Article 
650 4 |a carbon dots 
650 4 |a effective conjugation length 
650 4 |a light-emitting devices 
650 4 |a multiple-color emission 
650 4 |a phosphors 
700 1 |a Qu, Dan  |e verfasserin  |4 aut 
700 1 |a Yang, Dongxue  |e verfasserin  |4 aut 
700 1 |a Nie, Bing  |e verfasserin  |4 aut 
700 1 |a Zhao, Yikang  |e verfasserin  |4 aut 
700 1 |a Fan, Hongyou  |e verfasserin  |4 aut 
700 1 |a Sun, Zaicheng  |e verfasserin  |4 aut 
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856 4 0 |u http://dx.doi.org/10.1002/adma.201704740  |3 Volltext 
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