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231225s2018 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201704841
|2 doi
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|a pubmed24n0926.xml
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|a (DE-627)NLM27798078X
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|a (NLM)29131411
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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| 100 |
1 |
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|a Tong, Bo
|e verfasserin
|4 aut
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| 245 |
1 |
4 |
|a The Salt Matters
|b Enhanced Reversibility of Li-O2 Batteries with a Li[(CF3 SO2 )(n-C4 F9 SO2 )N]-Based Electrolyte
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|c 2018
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 01.08.2018
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a The safety hazards and cycle instability of lithium metal anodes (LMA) constitute significant barriers to progress in lithium metal batteries. This situation is worse in Li-O2 batteries because the LMA is prone to be chemically attacked by O2 shuttled from the cathode. Notwithstanding, efforts on LMA are much sparse than those on the cathode in the realm of Li-O2 batteries. Here, a novel lithium salt of Li[(CF3 SO2 )(n-C4 F9 SO2 )N] (LiTNFSI) is reported, which can effectively suppress the parasitic side reactions and dendrite growth of LMA during cycling and thereby significantly enhance the overall reversibility of Li-O2 batteries. A variety of advanced research tools are employed to scrutinize the working principles of the LiTNFSI salt. It is revealed that a stable, uniform, and O2 -resistive solid electrolyte interphase is formed on LMA, and hence the "cross-talk" between the LMA and O2 shuttled from the cathode is remarkably inhibited in LiTNFSI-based Li-O2 batteries
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|a Journal Article
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|a Li-O2 battery
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|a electrolyte engineering
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|a lithium metal anode
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4 |
|a reversibility
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| 650 |
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4 |
|a solid electrolyte interphase
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| 700 |
1 |
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|a Huang, Jun
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhou, Zhibin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Peng, Zhangquan
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 30(2018), 1 vom: 12. Jan.
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
1 |
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|g volume:30
|g year:2018
|g number:1
|g day:12
|g month:01
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|u http://dx.doi.org/10.1002/adma.201704841
|3 Volltext
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