Lateral Graphene-Contacted Vertically Stacked WS2 /MoS2 Hybrid Photodetectors with Large Gain

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 29(2017), 46 vom: 21. Dez.
1. Verfasser: Tan, Haijie (VerfasserIn)
Weitere Verfasser: Xu, Wenshuo, Sheng, Yuewen, Lau, Chit Siong, Fan, Ye, Chen, Qu, Tweedie, Martin, Wang, Xiaochen, Zhou, Yingqiu, Warner, Jamie H
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2017
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article MoS2 WS2 charge transfer heterostructures photodetectors
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520 |a A demonstration is presented of how significant improvements in all-2D photodetectors can be achieved by exploiting the type-II band alignment of vertically stacked WS2 /MoS2 semiconducting heterobilayers and finite density of states of graphene electrodes. The photoresponsivity of WS2 /MoS2 heterobilayer devices is increased by more than an order of magnitude compared to homobilayer devices and two orders of magnitude compared to monolayer devices of WS2 and MoS2 , reaching 103 A W-1 under an illumination power density of 1.7 × 102 mW cm-2 . The massive improvement in performance is due to the strong Coulomb interaction between WS2 and MoS2 layers. The efficient charge transfer at the WS2 /MoS2 heterointerface and long trapping time of photogenerated charges contribute to the observed large photoconductive gain of ≈3 × 104 . Laterally spaced graphene electrodes with vertically stacked 2D van der Waals heterostructures are employed for making high-performing ultrathin photodetectors 
650 4 |a Journal Article 
650 4 |a MoS2 
650 4 |a WS2 
650 4 |a charge transfer 
650 4 |a heterostructures 
650 4 |a photodetectors 
700 1 |a Xu, Wenshuo  |e verfasserin  |4 aut 
700 1 |a Sheng, Yuewen  |e verfasserin  |4 aut 
700 1 |a Lau, Chit Siong  |e verfasserin  |4 aut 
700 1 |a Fan, Ye  |e verfasserin  |4 aut 
700 1 |a Chen, Qu  |e verfasserin  |4 aut 
700 1 |a Tweedie, Martin  |e verfasserin  |4 aut 
700 1 |a Wang, Xiaochen  |e verfasserin  |4 aut 
700 1 |a Zhou, Yingqiu  |e verfasserin  |4 aut 
700 1 |a Warner, Jamie H  |e verfasserin  |4 aut 
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856 4 0 |u http://dx.doi.org/10.1002/adma.201702917  |3 Volltext 
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