|
|
|
|
| LEADER |
01000naa a22002652 4500 |
| 001 |
NLM275812510 |
| 003 |
DE-627 |
| 005 |
20231225010535.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231225s2017 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.201703601
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n0919.xml
|
| 035 |
|
|
|a (DE-627)NLM275812510
|
| 035 |
|
|
|a (NLM)28910497
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Wang, Zhili
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Tuning Surface Structure of 3D Nanoporous Gold by Surfactant-Free Electrochemical Potential Cycling
|
| 264 |
|
1 |
|c 2017
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Completed 18.07.2018
|
| 500 |
|
|
|a Date Revised 01.10.2020
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
|
| 520 |
|
|
|a 3D dealloyed nanoporous metals have emerged as a new class of catalysts for various chemical and electrochemical reactions. Similar to other heterogeneous catalysts, the surface atomic structure of the nanoporous metal catalysts plays a crucial role in catalytic activity and selectivity. Through surfactant-assisted bottom-up synthesis, the surface-structure modification has been successfully realized in low-dimensional particulate catalysts. However, the surface modification by top-down dealloying has not been well explored for nanoporous metal catalysts. Here, a surfactant-free approach to tailor the surface structure of nanoporous gold by surface relaxation via electrochemical redox cycling is reported. By controlling the scan rates, nanoporous gold with abundant {111} facets or {100} facets can be designed and fabricated with dramatically improved electrocatalysis toward the ethanol oxidation reaction
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a electrocatalysis
|
| 650 |
|
4 |
|a nanoporous gold
|
| 650 |
|
4 |
|a surface engineering
|
| 650 |
|
4 |
|a surface structure
|
| 700 |
1 |
|
|a Ning, Shoucong
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Liu, Pan
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Ding, Yi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Hirata, Akihiko
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Fujita, Takeshi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Chen, Mingwei
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 41 vom: 19. Nov.
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:29
|g year:2017
|g number:41
|g day:19
|g month:11
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.201703601
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 29
|j 2017
|e 41
|b 19
|c 11
|