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231225s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201701346
|2 doi
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|a pubmed24n0914.xml
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|a (DE-627)NLM274200686
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|a (NLM)28745406
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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| 100 |
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|a Park, Sang Kyu
|e verfasserin
|4 aut
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|a Highly Luminescent 2D-Type Slab Crystals Based on a Molecular Charge-Transfer Complex as Promising Organic Light-Emitting Transistor Materials
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 18.07.2018
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a A new 2:1 donor (D):acceptor (A) mixed-stacked charge-transfer (CT) cocrystal comprising isometrically structured dicyanodistyrylbenzene-based D and A molecules is designed and synthesized. Uniform 2D-type morphology is manifested by the exquisite interplay of intermolecular interactions. In addition to its appealing structural features, unique optoelectronic properties are unveiled. Exceptionally high photoluminescence quantum yield (ΦF ≈ 60%) is realized by non-negligible oscillator strength of the S1 transition, and rigidified 2D-type structure. Moreover, this luminescent 2D-type CT crystal exhibits balanced ambipolar transport (µh and µe of ≈10-4 cm2 V-1 s-1 ). As a consequence of such unique optoelectronic characteristics, the first CT electroluminescence is demonstrated in a single active-layered organic light-emitting transistor (OLET) device. The external quantum efficiency of this OLET is as high as 1.5% to suggest a promising potential of luminescent mixed-stacked CT cocrystals in OLET applications
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|a Journal Article
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|a 2D
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|a ambipolar transport
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|a charge-transfer complexes
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|a luminescence
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|a organic light-emitting transistors
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|a Kim, Jin Hong
|e verfasserin
|4 aut
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|a Ohto, Tatsuhiko
|e verfasserin
|4 aut
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|a Yamada, Ryo
|e verfasserin
|4 aut
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|a Jones, Andrew O F
|e verfasserin
|4 aut
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|a Whang, Dong Ryeol
|e verfasserin
|4 aut
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|a Cho, Illhun
|e verfasserin
|4 aut
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|a Oh, Sangyoon
|e verfasserin
|4 aut
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|a Hong, Seung Hwa
|e verfasserin
|4 aut
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|a Kwon, Ji Eon
|e verfasserin
|4 aut
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|a Kim, Jong H
|e verfasserin
|4 aut
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|a Olivier, Yoann
|e verfasserin
|4 aut
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|a Fischer, Roland
|e verfasserin
|4 aut
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|a Resel, Roland
|e verfasserin
|4 aut
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|a Gierschner, Johannes
|e verfasserin
|4 aut
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|a Tada, Hirokazu
|e verfasserin
|4 aut
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|a Park, Soo Young
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 36 vom: 10. Sept.
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:29
|g year:2017
|g number:36
|g day:10
|g month:09
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|u http://dx.doi.org/10.1002/adma.201701346
|3 Volltext
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