Spatially Resolved Large Magnetization in Ultrathin BiFeO3

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 29(2017), 32 vom: 04. Aug.
1. Verfasser: Guo, Er-Jia (VerfasserIn)
Weitere Verfasser: Petrie, Jonathan R, Roldan, Manuel A, Li, Qian, Desautels, Ryan D, Charlton, Timothy, Herklotz, Andreas, Nichols, John, van Lierop, Johan, Freeland, John W, Kalinin, Sergei V, Lee, Ho Nyung, Fitzsimmons, Michael R
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2017
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article X-ray absorption complex oxide superlattice multiferroic polarized neutron reflectometry
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245 1 0 |a Spatially Resolved Large Magnetization in Ultrathin BiFeO3 
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520 |a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. 
520 |a Here, a quantitative magnetic depth profile across the planar interfaces in BiFeO3 /La0.7 Sr0.3 MnO3 (BFO/LSMO) superlattices using polarized neutron reflectometry is obtained. An enhanced magnetization of 1.83 ± 0.16 μB /Fe in BFO layers is observed when they are interleaved between two manganite layers. The enhanced magnetic order in BFO persists up to 200 K. The depth dependence of magnetic moments in BFO/LSMO superlattices as a function of the BFO layer thickness is also explored. The results show the enhanced net magnetic moment in BFO from the LSMO/BFO interface extends 3-4 unit cells into BFO. The interior part of a thicker BFO layer has a much smaller magnetization, suggesting it still keeps the small canted AFM state. The results exclude charge transfer, intermixing, epitaxial strain, and octahedral rotations/tilts as dominating mechanisms for the large net magnetization in BFO. An explanation-one suggested by others previously and consistent with the observations-attributes the temperature dependence of the net magnetization of BFO to strong orbital hybridization between Fe and Mn across the interfaces. Such orbital reconstruction would establish an upper temperature limit for magnetic ordering of BFO 
650 4 |a Journal Article 
650 4 |a X-ray absorption 
650 4 |a complex oxide superlattice 
650 4 |a multiferroic 
650 4 |a polarized neutron reflectometry 
700 1 |a Petrie, Jonathan R  |e verfasserin  |4 aut 
700 1 |a Roldan, Manuel A  |e verfasserin  |4 aut 
700 1 |a Li, Qian  |e verfasserin  |4 aut 
700 1 |a Desautels, Ryan D  |e verfasserin  |4 aut 
700 1 |a Charlton, Timothy  |e verfasserin  |4 aut 
700 1 |a Herklotz, Andreas  |e verfasserin  |4 aut 
700 1 |a Nichols, John  |e verfasserin  |4 aut 
700 1 |a van Lierop, Johan  |e verfasserin  |4 aut 
700 1 |a Freeland, John W  |e verfasserin  |4 aut 
700 1 |a Kalinin, Sergei V  |e verfasserin  |4 aut 
700 1 |a Lee, Ho Nyung  |e verfasserin  |4 aut 
700 1 |a Fitzsimmons, Michael R  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Advanced materials (Deerfield Beach, Fla.)  |d 1998  |g 29(2017), 32 vom: 04. Aug.  |w (DE-627)NLM098206397  |x 1521-4095  |7 nnns 
773 1 8 |g volume:29  |g year:2017  |g number:32  |g day:04  |g month:08 
856 4 0 |u http://dx.doi.org/10.1002/adma.201700790  |3 Volltext 
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