In Situ Electrochemistry of Rechargeable Battery Materials : Status Report and Perspectives

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 29(2017), 31 vom: 10. Aug.
1. Verfasser: Yang, Yijun (VerfasserIn)
Weitere Verfasser: Liu, Xizheng, Dai, Zhonghua, Yuan, Fangli, Bando, Yoshio, Golberg, Dmitri, Wang, Xi
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2017
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article Review in situ electrochemical rechargeable batteries structure evolution surface/interface changes
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520 |a The development of rechargeable batteries with high performance is considered to be a feasible way to satisfy the increasing needs of electric vehicles and portable devices. It is of vital importance to design electrodes with high electrochemical performance and to understand the nature of the electrode/electrolyte interfaces during battery operation, which allows a direct observation of the complicated chemical and physical processes within the electrodes and electrolyte, and thus provides real-time information for further design and optimization of the battery performance. Here, the recent progress in in situ techniques employed for the investigations of material structural evolutions is described, including characterization using neutrons, X-ray diffraction, and nuclear magnetic resonance. In situ techniques utilized for in-depth uncovering the electrode/electrolyte phase/interface change mechanisms are then highlighted, including transmission electron microscopy, atomic force microscopy, X-ray spectroscopy, and Raman spectroscopy. The real-time monitoring of lithium dendrite growth and in situ detection of gas evolution during charge/discharge processes are also discussed. Finally, the major challenges and opportunities of in situ characterization techniques are outlined toward new developments of rechargeable batteries, including innovation in the design of compatible in situ cells, applications of dynamic analysis, and in situ electrochemistry under multi-stimuli. A clear and in-depth understanding of in situ technique applications and the mechanisms of structural evolutions, surface/interface changes, and gas generations within rechargeable batteries is given here 
650 4 |a Journal Article 
650 4 |a Review 
650 4 |a in situ electrochemical 
650 4 |a rechargeable batteries 
650 4 |a structure evolution 
650 4 |a surface/interface changes 
700 1 |a Liu, Xizheng  |e verfasserin  |4 aut 
700 1 |a Dai, Zhonghua  |e verfasserin  |4 aut 
700 1 |a Yuan, Fangli  |e verfasserin  |4 aut 
700 1 |a Bando, Yoshio  |e verfasserin  |4 aut 
700 1 |a Golberg, Dmitri  |e verfasserin  |4 aut 
700 1 |a Wang, Xi  |e verfasserin  |4 aut 
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