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231224s2017 xx |||||o 00| ||eng c |
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7 |
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|a 10.1002/adma.201606357
|2 doi
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|a pubmed24n0906.xml
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|a eng
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| 100 |
1 |
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|a Sitaputra, Wattaka
|e verfasserin
|4 aut
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| 245 |
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|a In Situ Probing of Ion Ordering at an Electrified Ionic Liquid/Au Interface
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Completed 18.07.2018
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Charge transport at the interface of electrodes and ionic liquids is critical for the use of the latter as electrolytes. A room-temperature ionic liquid, 1-ethyl-2,3-dimethylimidazolium bis(trifluoromethanesulfonyl)imide (EMMIM TFSI), is investigated in situ under applied bias voltage with a novel method using low-energy electron and photoemission electron microscopy. Changes in photoelectron yield as a function of bias applied to electrodes provide a direct measure of the dynamics of ion reconfiguration and electrostatic responses of the EMMIM TFSI. Long-range and correlated ionic reconfigurations that occur near the electrodes are found to be a function of temperature and thickness, which, in turn, relate to ionic mobility and different configurations for out-of-plane ordering near the electrode interfaces, with a critical transition in ion mobility for films thicker than three monolayers
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|a Journal Article
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|a electric double layers
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4 |
|a ionic liquids
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| 650 |
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4 |
|a photoemission electron microscopy
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1 |
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|a Stacchiola, Dario
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wishart, James F
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wang, Feng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Sadowski, Jerzy T
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 27 vom: 01. Juli
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|x 1521-4095
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|g volume:29
|g year:2017
|g number:27
|g day:01
|g month:07
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|u http://dx.doi.org/10.1002/adma.201606357
|3 Volltext
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