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231224s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201700274
|2 doi
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|a pubmed25n0904.xml
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|a (NLM)28452147
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|a DE-627
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|e rakwb
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|a eng
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|a Zeng, Yinxiang
|e verfasserin
|4 aut
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|a Achieving Ultrahigh Energy Density and Long Durability in a Flexible Rechargeable Quasi-Solid-State Zn-MnO2 Battery
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 18.07.2018
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Advanced flexible batteries with high energy density and long cycle life are an important research target. Herein, the first paradigm of a high-performance and stable flexible rechargeable quasi-solid-state Zn-MnO2 battery is constructed by engineering MnO2 electrodes and gel electrolyte. Benefiting from a poly(3,4-ethylenedioxythiophene) (PEDOT) buffer layer and a Mn2+ -based neutral electrolyte, the fabricated Zn-MnO2 PEDOT battery presents a remarkable capacity of 366.6 mA h g-1 and good cycling performance (83.7% after 300 cycles) in aqueous electrolyte. More importantly, when using PVA/ZnCl2 /MnSO4 gel as electrolyte, the as-fabricated quasi-solid-state Zn-MnO2 @PEDOT battery remains highly rechargeable, maintaining more than 77.7% of its initial capacity and nearly 100% Coulombic efficiency after 300 cycles. Moreover, this flexible quasi-solid-state Zn-MnO2 battery achieves an admirable energy density of 504.9 W h kg-1 (33.95 mW h cm-3 ), together with a peak power density of 8.6 kW kg-1 , substantially higher than most recently reported flexible energy-storage devices. With the merits of impressive energy density and durability, this highly flexible rechargeable Zn-MnO2 battery opens new opportunities for powering portable and wearable electronics
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|a Journal Article
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|a Zn-MnO2 batteries
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|a durability
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|a flexible
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|a rechargeable
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|a ultrahigh energy density
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|a Zhang, Xiyue
|e verfasserin
|4 aut
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|a Meng, Yue
|e verfasserin
|4 aut
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|a Yu, Minghao
|e verfasserin
|4 aut
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|a Yi, Jianan
|e verfasserin
|4 aut
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|a Wu, Yiqiang
|e verfasserin
|4 aut
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|a Lu, Xihong
|e verfasserin
|4 aut
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|a Tong, Yexiang
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 26 vom: 01. Juli
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:29
|g year:2017
|g number:26
|g day:01
|g month:07
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|u http://dx.doi.org/10.1002/adma.201700274
|3 Volltext
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