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231224s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201606831
|2 doi
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|a pubmed24n0903.xml
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|a (DE-627)NLM271045566
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|a (NLM)28417505
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|a DE-627
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|c DE-627
|e rakwb
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|a eng
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|a Kim, Dong Hoe
|e verfasserin
|4 aut
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|a 300% Enhancement of Carrier Mobility in Uniaxial-Oriented Perovskite Films Formed by Topotactic-Oriented Attachment
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 18.07.2018
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Organic-inorganic perovskites with intriguing optical and electrical properties have attracted significant research interests due to their excellent performance in optoelectronic devices. Recent efforts on preparing uniform and large-grain polycrystalline perovskite films have led to enhanced carrier lifetime up to several microseconds. However, the mobility and trap densities of polycrystalline perovskite films are still significantly behind their single-crystal counterparts. Here, a facile topotactic-oriented attachment (TOA) process to grow highly oriented perovskite films, featuring strong uniaxial-crystallographic texture, micrometer-grain morphology, high crystallinity, low trap density (≈4 × 1014 cm-3 ), and unprecedented 9 GHz charge-carrier mobility (71 cm2 V-1 s-1 ), is demonstrated. TOA-perovskite-based n-i-p planar solar cells show minimal discrepancies between stabilized efficiency (19.0%) and reverse-scan efficiency (19.7%). The TOA process is also applicable for growing other state-of-the-art perovskite alloys, including triple-cation and mixed-halide perovskites
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|a Journal Article
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|a carrier mobility
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|a orientation
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|a perovskite films
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|a solar cells
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|a topotactic-oriented attachment
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|a Park, Jaehong
|e verfasserin
|4 aut
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|a Li, Zhen
|e verfasserin
|4 aut
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|a Yang, Mengjin
|e verfasserin
|4 aut
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|a Park, Ji-Sang
|e verfasserin
|4 aut
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|a Park, Ik Jae
|e verfasserin
|4 aut
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|a Kim, Jin Young
|e verfasserin
|4 aut
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|a Berry, Joseph J
|e verfasserin
|4 aut
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|a Rumbles, Garry
|e verfasserin
|4 aut
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|a Zhu, Kai
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 23 vom: 20. Juni
|w (DE-627)NLM098206397
|x 1521-4095
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|g volume:29
|g year:2017
|g number:23
|g day:20
|g month:06
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|u http://dx.doi.org/10.1002/adma.201606831
|3 Volltext
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