Pt/ZnOC Nanocable with Dual-Enhanced Photocatalytic Performance and Superior Photostability
To improve the photocatalytic activity and photostability of ZnO, a novel cable-like Pt/ZnOC composite is successfully fabricated by coating a 3-5 nm hydrothermal carbon (HTC) layer on the surface of the Pt nanoparticle-modified ZnO nanowire. After investigating the optical and photoelectrochemical...
| Publié dans: | Langmuir : the ACS journal of surfaces and colloids. - 1985. - 33(2017), 18 vom: 09. Mai, Seite 4452-4460 |
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| Auteur principal: | |
| Autres auteurs: | , , , , , , |
| Format: | Article en ligne |
| Langue: | English |
| Publié: |
2017
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| Accès à la collection: | Langmuir : the ACS journal of surfaces and colloids |
| Sujets: | Journal Article Research Support, Non-U.S. Gov't |
| Résumé: | To improve the photocatalytic activity and photostability of ZnO, a novel cable-like Pt/ZnOC composite is successfully fabricated by coating a 3-5 nm hydrothermal carbon (HTC) layer on the surface of the Pt nanoparticle-modified ZnO nanowire. After investigating the optical and photoelectrochemical performance in detail, it is found that the Pt/ZnO@C nanocable shows a dual-enhanced migration efficiency for the photoinduced surface electrons, distributing to the modified Pt nanoparticles and the coated HTC layer. Consequently, the Pt/ZnO@C nanocable exhibits a dual-enhanced photocatalytic activity for the degradation of various organic pollutants under the UV light irradiation. The coated HTC layer can also play a role in suspending the ZnO photocorrosion and significantly improves the photostability of the Pt/ZnO@C nanocable. Furthermore, the photocatalysis and photocorrosion mechanism of the Pt/ZnO@C nanocable is proposed and discussed in terms of its structural feature and photoelectrochemical property. The resultant Pt/ZnO@C nanocable with the unique HTC layer-coated structure will probably stimulate to design and synthesize more HTC-hybridized composites with a superior photocatalytic or photoelectrocatalytic performance |
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| Description: | Date Completed 10.07.2018 Date Revised 10.07.2018 published: Print-Electronic Citation Status PubMed-not-MEDLINE |
| ISSN: | 1520-5827 |
| DOI: | 10.1021/acs.langmuir.7b00995 |