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231224s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201700008
|2 doi
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|a eng
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| 100 |
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|a Ou, Honghui
|e verfasserin
|4 aut
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|a Tri-s-triazine-Based Crystalline Carbon Nitride Nanosheets for an Improved Hydrogen Evolution
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|c 2017
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|a Text
|b txt
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Completed 18.07.2018
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Tri-s-triazine-based crystalline carbon nitride nanosheets (CCNNSs) have been successfully extracted via a conventional and cost-effective sonication-centrifugation process. These CCNNSs possess a highly defined and unambiguous structure with minimal thickness, large aspect ratios, homogeneous tri-s-triazine-based units, and high crystallinity. These tri-s-triazine-based CCNNSs show significantly enhanced photocatalytic hydrogen generation activity under visible light than g-C3 N4 , poly (triazine imide)/Li+ Cl- , and bulk tri-s-triazine-based crystalline carbon nitrides. A highly apparent quantum efficiency of 8.57% at 420 nm for hydrogen production from aqueous methanol feedstock can be achieved from tri-s-triazine-based CCNNSs, exceeding most of the reported carbon nitride nanosheets. Benefiting from the inherent structure of 2D crystals, the ultrathin tri-s-triazine-based CCNNSs provide a broad range of application prospects in the fields of bioimaging, and energy storage and conversion
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|a Journal Article
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|a crystalline carbon nitride
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|a few-layered nanosheets
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|a hydrogen evolution
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|a photocatalysis
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|a tri-s-triazine
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1 |
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|a Lin, Lihua
|e verfasserin
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| 700 |
1 |
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|a Zheng, Yun
|e verfasserin
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| 700 |
1 |
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|a Yang, Pengju
|e verfasserin
|4 aut
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1 |
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|a Fang, Yuanxing
|e verfasserin
|4 aut
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| 700 |
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|a Wang, Xinchen
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 22 vom: 01. Juni
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|u http://dx.doi.org/10.1002/adma.201700008
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