Trap Healing for High-Performance Low-Voltage Polymer Transistors and Solution-Based Analog Amplifiers on Foil

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 29(2017), 23 vom: 07. Juni
1. Verfasser: Pecunia, Vincenzo (VerfasserIn)
Weitere Verfasser: Nikolka, Mark, Sou, Antony, Nasrallah, Iyad, Amin, Atefeh Y, McCulloch, Iain, Sirringhaus, Henning
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2017
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article charge trapping low-voltage amplifiers low-voltage polymer transistors solution-based integration
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500 |a Date Completed 18.07.2018 
500 |a Date Revised 30.09.2020 
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520 |a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. 
520 |a Solution-processed semiconductors such as conjugated polymers have great potential in large-area electronics. While extremely appealing due to their low-temperature and high-throughput deposition methods, their integration in high-performance circuits has been difficult. An important remaining challenge is the achievement of low-voltage circuit operation. The present study focuses on state-of-the-art polymer thin-film transistors based on poly(indacenodithiophene-benzothiadiazole) and shows that the general paradigm for low-voltage operation via an enhanced gate-to-channel capacitive coupling is unable to deliver high-performance device behavior. The order-of-magnitude longitudinal-field reduction demanded by low-voltage operation plays a fundamental role, enabling bulk trapping and leading to compromised contact properties. A trap-reduction technique based on small molecule additives, however, is capable of overcoming this effect, allowing low-voltage high-mobility operation. This approach is readily applicable to low-voltage circuit integration, as this work exemplifies by demonstrating high-performance analog differential amplifiers operating at a battery-compatible power supply voltage of 5 V with power dissipation of 11 µW, and attaining a voltage gain above 60 dB at a power supply voltage below 8 V. These findings constitute an important milestone in realizing low-voltage polymer transistors for solution-based analog electronics that meets performance and power-dissipation requirements for a range of battery-powered smart-sensing applications 
650 4 |a Journal Article 
650 4 |a charge trapping 
650 4 |a low-voltage amplifiers 
650 4 |a low-voltage polymer transistors 
650 4 |a solution-based integration 
700 1 |a Nikolka, Mark  |e verfasserin  |4 aut 
700 1 |a Sou, Antony  |e verfasserin  |4 aut 
700 1 |a Nasrallah, Iyad  |e verfasserin  |4 aut 
700 1 |a Amin, Atefeh Y  |e verfasserin  |4 aut 
700 1 |a McCulloch, Iain  |e verfasserin  |4 aut 
700 1 |a Sirringhaus, Henning  |e verfasserin  |4 aut 
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773 1 8 |g volume:29  |g year:2017  |g number:23  |g day:07  |g month:06 
856 4 0 |u http://dx.doi.org/10.1002/adma.201606938  |3 Volltext 
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