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231224s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201606938
|2 doi
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|a pubmed24n0902.xml
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|a (NLM)28397305
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|a DE-627
|b ger
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|e rakwb
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|a eng
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|a Pecunia, Vincenzo
|e verfasserin
|4 aut
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|a Trap Healing for High-Performance Low-Voltage Polymer Transistors and Solution-Based Analog Amplifiers on Foil
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 18.07.2018
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Solution-processed semiconductors such as conjugated polymers have great potential in large-area electronics. While extremely appealing due to their low-temperature and high-throughput deposition methods, their integration in high-performance circuits has been difficult. An important remaining challenge is the achievement of low-voltage circuit operation. The present study focuses on state-of-the-art polymer thin-film transistors based on poly(indacenodithiophene-benzothiadiazole) and shows that the general paradigm for low-voltage operation via an enhanced gate-to-channel capacitive coupling is unable to deliver high-performance device behavior. The order-of-magnitude longitudinal-field reduction demanded by low-voltage operation plays a fundamental role, enabling bulk trapping and leading to compromised contact properties. A trap-reduction technique based on small molecule additives, however, is capable of overcoming this effect, allowing low-voltage high-mobility operation. This approach is readily applicable to low-voltage circuit integration, as this work exemplifies by demonstrating high-performance analog differential amplifiers operating at a battery-compatible power supply voltage of 5 V with power dissipation of 11 µW, and attaining a voltage gain above 60 dB at a power supply voltage below 8 V. These findings constitute an important milestone in realizing low-voltage polymer transistors for solution-based analog electronics that meets performance and power-dissipation requirements for a range of battery-powered smart-sensing applications
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|a Journal Article
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|a charge trapping
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|a low-voltage amplifiers
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|a low-voltage polymer transistors
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|a solution-based integration
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|a Nikolka, Mark
|e verfasserin
|4 aut
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|a Sou, Antony
|e verfasserin
|4 aut
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|a Nasrallah, Iyad
|e verfasserin
|4 aut
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|a Amin, Atefeh Y
|e verfasserin
|4 aut
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|a McCulloch, Iain
|e verfasserin
|4 aut
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|a Sirringhaus, Henning
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 23 vom: 07. Juni
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:29
|g year:2017
|g number:23
|g day:07
|g month:06
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|u http://dx.doi.org/10.1002/adma.201606938
|3 Volltext
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