High-Efficiency Photovoltaic Devices using Trap-Controlled Quantum-Dot Ink prepared via Phase-Transfer Exchange

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 29(2017), 19 vom: 11. Mai
1. Verfasser: Aqoma, Havid (VerfasserIn)
Weitere Verfasser: Al Mubarok, Muhibullah, Hadmojo, Wisnu Tantyo, Lee, Eun-Hye, Kim, Tae-Wook, Ahn, Tae Kyu, Oh, Seung-Hwan, Jang, Sung-Yeon
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2017
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article phase-transfer exchange quantum dots solar cells surface traps voltage loss
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500 |a Date Completed 18.07.2018 
500 |a Date Revised 30.09.2020 
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520 |a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. 
520 |a Colloidal-quantum-dot (CQD) photovoltaic devices are promising candidates for low-cost power sources owing to their low-temperature solution processability and bandgap tunability. A power conversion efficiency (PCE) of >10% is achieved for these devices; however, there are several remaining obstacles to their commercialization, including their high energy loss due to surface trap states and the complexity of the multiple-step CQD-layer-deposition process. Herein, high-efficiency photovoltaic devices prepared with CQD-ink using a phase-transfer-exchange (PTE) method are reported. Using CQD-ink, the fabrication of active layers by single-step coating and the suppression of surface trap states are achieved simultaneously. The CQD-ink photovoltaic devices achieve much higher PCEs (10.15% with a certified PCE of 9.61%) than the control devices (7.85%) owing to improved charge drift and diffusion. Notably, the CQD-ink devices show much lower energy loss than other reported high-efficiency CQD devices. This result reveals that the PTE method is an effective strategy for controlling trap states in CQDs 
650 4 |a Journal Article 
650 4 |a phase-transfer exchange 
650 4 |a quantum dots 
650 4 |a solar cells 
650 4 |a surface traps 
650 4 |a voltage loss 
700 1 |a Al Mubarok, Muhibullah  |e verfasserin  |4 aut 
700 1 |a Hadmojo, Wisnu Tantyo  |e verfasserin  |4 aut 
700 1 |a Lee, Eun-Hye  |e verfasserin  |4 aut 
700 1 |a Kim, Tae-Wook  |e verfasserin  |4 aut 
700 1 |a Ahn, Tae Kyu  |e verfasserin  |4 aut 
700 1 |a Oh, Seung-Hwan  |e verfasserin  |4 aut 
700 1 |a Jang, Sung-Yeon  |e verfasserin  |4 aut 
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773 1 8 |g volume:29  |g year:2017  |g number:19  |g day:11  |g month:05 
856 4 0 |u http://dx.doi.org/10.1002/adma.201605756  |3 Volltext 
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