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231224s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201605756
|2 doi
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|a pubmed24n0898.xml
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|a (DE-627)NLM269580735
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|a (NLM)28266746
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Aqoma, Havid
|e verfasserin
|4 aut
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|a High-Efficiency Photovoltaic Devices using Trap-Controlled Quantum-Dot Ink prepared via Phase-Transfer Exchange
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 18.07.2018
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Colloidal-quantum-dot (CQD) photovoltaic devices are promising candidates for low-cost power sources owing to their low-temperature solution processability and bandgap tunability. A power conversion efficiency (PCE) of >10% is achieved for these devices; however, there are several remaining obstacles to their commercialization, including their high energy loss due to surface trap states and the complexity of the multiple-step CQD-layer-deposition process. Herein, high-efficiency photovoltaic devices prepared with CQD-ink using a phase-transfer-exchange (PTE) method are reported. Using CQD-ink, the fabrication of active layers by single-step coating and the suppression of surface trap states are achieved simultaneously. The CQD-ink photovoltaic devices achieve much higher PCEs (10.15% with a certified PCE of 9.61%) than the control devices (7.85%) owing to improved charge drift and diffusion. Notably, the CQD-ink devices show much lower energy loss than other reported high-efficiency CQD devices. This result reveals that the PTE method is an effective strategy for controlling trap states in CQDs
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|a Journal Article
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|a phase-transfer exchange
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|a quantum dots
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|a solar cells
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|a surface traps
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|a voltage loss
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|a Al Mubarok, Muhibullah
|e verfasserin
|4 aut
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|a Hadmojo, Wisnu Tantyo
|e verfasserin
|4 aut
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|a Lee, Eun-Hye
|e verfasserin
|4 aut
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|a Kim, Tae-Wook
|e verfasserin
|4 aut
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|a Ahn, Tae Kyu
|e verfasserin
|4 aut
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|a Oh, Seung-Hwan
|e verfasserin
|4 aut
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|a Jang, Sung-Yeon
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 19 vom: 11. Mai
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:29
|g year:2017
|g number:19
|g day:11
|g month:05
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|u http://dx.doi.org/10.1002/adma.201605756
|3 Volltext
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