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231224s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201606688
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|a pubmed24n0898.xml
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|a (NLM)28262995
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|a DE-627
|b ger
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|e rakwb
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|a eng
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|a Zhang, Zhenyi
|e verfasserin
|4 aut
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|a A Nonmetal Plasmonic Z-Scheme Photocatalyst with UV- to NIR-Driven Photocatalytic Protons Reduction
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|c 2017
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|a Text
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Completed 18.07.2018
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|a Date Revised 30.09.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a Ultrabroad-spectrum absorption and highly efficient generation of available charge carriers are two essential requirements for promising semiconductor-based photocatalysts, towards achieving the ultimate goal of solar-to-fuel conversion. Here, a fascinating nonmetal plasmonic Z-scheme photocatalyst with the W18 O49 /g-C3 N4 heterostructure is reported, which can effectively harvest photon energies spanning from the UV to the nearinfrared region and simultaneously possesses improved charge-carrier dynamics to boost the generation of long-lived active electrons for the photocatalytic reduction of protons into H2 . By combining with theoretical simulations, a unique synergistic photocatalysis effect between the semiconductive Z-scheme charge-carrier separation and metal-like localized-surface-plasmon-resonance-induced "hot electrons" injection process is demonstrated within this binary heterostructure
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|a Journal Article
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|a H2 evolution
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|a Z-scheme photocatalysts
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|a full-solar-spectrum absorption
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|a photocatalysis
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|a plasmonic semiconductors
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|a Huang, Jindou
|e verfasserin
|4 aut
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|a Fang, Yurui
|e verfasserin
|4 aut
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|a Zhang, Mingyi
|e verfasserin
|4 aut
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|a Liu, Kuichao
|e verfasserin
|4 aut
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|a Dong, Bin
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 18 vom: 06. Mai
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:29
|g year:2017
|g number:18
|g day:06
|g month:05
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|u http://dx.doi.org/10.1002/adma.201606688
|3 Volltext
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