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231224s2016 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.6b01594
|2 doi
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|a eng
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| 100 |
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|a Zhu, Genxing
|e verfasserin
|4 aut
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| 245 |
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|a Evolution from Classical to Non-classical Aggregation-Based Crystal Growth of Calcite by Organic Additive Control
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|c 2016
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|a Text
|b txt
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|a ƒaComputermedien
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|a Date Completed 01.06.2018
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|a Date Revised 01.06.2018
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a Aggregation-based crystal growth is distinct from the classical understanding of solution crystallization. In this study, we reveal that N-stearoyl-l-glutamic acid (C18-Glu, an amphiphile that mimics a biomineralization-relevant biomolecule) can switch calcite crystallization from a classical ion-by-ion growth to a non-classical particle-by-particle pathway, which combines the classical and non-classical crystallization in one system. This growth mechanism change is controlled by the concentration ratio of [C18-Glu]/[Ca(2+)] in solution. The high [C18-Glu]/[Ca(2+)] can stabilize precursor nanoparticles to provide building blocks for aggregation-based crystallization, in which the interaction between C18-Glu and the nanoprecursor phase rather than that of C18-Glu on calcite steps is highlighted. Our finding emphasizes the enrollment of organic additives on metastable nano building blocks, which provides an alternative understanding about organic control in inorganic crystallization
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|a Journal Article
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|a Research Support, Non-U.S. Gov't
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|a Yao, Shasha
|e verfasserin
|4 aut
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|a Zhai, Halei
|e verfasserin
|4 aut
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| 700 |
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|a Liu, Zhaoming
|e verfasserin
|4 aut
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|a Li, Yaling
|e verfasserin
|4 aut
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|a Pan, Haihua
|e verfasserin
|4 aut
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|a Tang, Ruikang
|e verfasserin
|4 aut
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1992
|g 32(2016), 35 vom: 06. Sept., Seite 8999-9004
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|x 1520-5827
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|g volume:32
|g year:2016
|g number:35
|g day:06
|g month:09
|g pages:8999-9004
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