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231224s2016 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.6b01536
|2 doi
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|a eng
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|a Martin, Elizabeth J
|e verfasserin
|4 aut
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|a Anodic Electrodeposition of a Cationic Polyelectrolyte in the Presence of Multivalent Anions
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|c 2016
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|a Text
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|a ƒaComputermedien
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|a Date Completed 30.05.2018
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|a Date Revised 30.05.2018
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a The electrochemical quartz crystal microbalance (QCM) was used to investigate the deposition of poly(allylamine hydrochloride) (PAH) with molybdate anions under anodic conditions. The PAH-molybdate complex was used as a model system to understand possible deposition criteria which may be relevant to the formation of proteinaceous films on CoCrMo hip implants. Data indicate that PAH deposition will occur above ∼0.60 V vs SCE if molybdate anions are present in the electrolyte above a critical concentration, and if the polymer concentration remains below a critical value. Numerical modeling and dynamic light scattering (DLS) studies were performed to understand the conditions that enable deposition to occur at these potentials. The results indicate that PAH-molybdate complexes form most efficiently when the polyvalent positive charge and polyvalent negative charge in the system are in an optimum range with respect to each other
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|a Journal Article
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|a Research Support, U.S. Gov't, Non-P.H.S.
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|a Sadman, Kazi
|e verfasserin
|4 aut
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|a Shull, Kenneth R
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1985
|g 32(2016), 31 vom: 09. Aug., Seite 7747-56
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|g year:2016
|g number:31
|g day:09
|g month:08
|g pages:7747-56
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